SYSTEM SIMULATION OF SPACEBORNE AND AIRBORNE HIGH SPECTRAL RESOLUTION LIDAR FOR AEROSOL MONITORING

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SYSTEM SIMULATION OF SPACEBORNE AND AIRBORNE HIGH SPECTRAL RESOLUTION LIDAR FOR AEROSOL MONITORING X. Wang 1, C. Song 2, A. Boselli 3, M. Iarlori 4, V. Rizi 4, N. Spinelli 2 changbo.song@unina.it CNISM-BRIT China-Italy Joint Research Center for Laser Remote Sensing and 1CNR-SPIN, Napoli, Italy 2 Dipartimento di Fisica, Università degli Studi di Napoli Federico II, Napoli, Italy 3CNR-IMAA, Potenza, Italy 4 CETEMPS, Dipartimento di Scienze Fisiche e Chimiche, Università degli Studi dell Aquila, L Aquila, Italy Abstract: Atmospheric aerosols play very important roles in climate change and air particulate pollution. Due to their highly variable optical and physical properties as well as to short atmospheric lifetimes and large spatial and temporal gradients, the aerosol impact on climate models and air pollution is really a complex task. Lidars based on elastic scattering have been largely used to measure aerosol spatial distribution and to derive their properties, but elastic backscatter Lidar data require the assumption of the aerosol extinction-to-backscatter ratio to retrieve aerosol optical properties profiles. To overcome this disadvantage, two main methods, High Spectral Resolution Lidar (HSRL) and Raman lidar, can be used to measure aerosol optical properties without a-priori hypotheses. Compared to Raman lidar, HSRL has the advantage of day and night measurements and can be adapted to many kinds of carrying platforms. HSRL can provide the vertical profile of aerosol extinction by separating the Mie signal by atmospheric aerosol and the Rayleigh signal by atmospheric molecules. Due to small spectral difference between Mie and Rayleigh signals, there are three difficulties: firstly, the laser source must have a narrow bandwidth, high energy and stable center wavelength; secondly, the receiver should have a very narrow spectral filter to separate aerosol scattering and molecular scattering; thirdly, the center wavelength of the receiver must be real-time locked to laser source. In order to study the influence of system parameters and to optimize their values, a system simulation of high spectral resolution lidar for aerosol monitoring has been done and will be presented in this paper.

1. Introduction Atmospheric aerosols influence the radiative budget of the earth directly through scattering and absorbtion of solar radiation and indirectly as cloud condensation nuclei. Regarding the accounting for direct and indirect aerosol radiative effects on climate change, the Intergovernmental Panel on Climate Change concluded that the uncertainties associated with the aerosol radiative forcing are larger than the uncertainties associated with any of the other principal components having a role in the climate change (http://www.ipcc.ch/report/ar5/wg1/). Due to the highly variable optical and physical properties as well as to the short atmospheric lifetimes and large spatial and temporal gradients it is really a complex task to evaluate the aerosol radiative forcing impact on climate models. Therefore, accurate measurements of aerosol optical properties and vertical profile are very important. The lidar technique has proved to be effective to measure the vertical profile of aerosol optical properties with high spatial and temporal resolution. However, a standard backscatter lidar can t obtain aerosol backscattering and extinction coefficients directly. The retrieval of both particulate extinction and backscatter coefficients relies on an assumption of a value for the extinction to backscattering ratio, the lidar ratio. But the actual value of the lidar ratio depends on the particle composition, size distribution, and shape. It can vary widely and, for any given observation or scene, can be difficult to estimate [1]. In order to obtain aerosol optical properties without a-priori hypotheses two main methods, High Spectral Resolution Lidar (HSRL) and Raman lidar, can be used. With these methods, the aerosol characteristics can be retrieved without assumptions on the aerosol extinction-to-backscatter ratio, offering both high vertical and temporal resolution. In particular the HSRL has the advantage of day and night measurements and can be adapted to many kinds of carrying platforms. Ground HSRL has been built at Montana State University [2] and airborne HSRL has been used to measure aerosol optical properties by Langley Research Center, NASA [1]. HSRL can provide the vertical profile of aerosol extinction by separating the Mie signal by atmospheric aerosol from Rayleigh signal by atmospheric molecules. The optimization of the systems parameters of the high spectral resolution lidar for aerosol monitoring has been studied by means of a system simulation. The system simulation method and result will be presented. 2. System schematic and simulation method High spectral resolution lidars (HSRLs) use a narrow-band optical filter to separate light that has been scattered by atmospheric aerosols from light that has been scattered by atmospheric molecules. This is possible because the light scattered by molecules differs spectrally from that scattered by aerosols [1]. Due to the thermal motion of the air molecules, light that has been scattered by molecules experiences a larger Doppler broadening with respect to light that has been scattered by atmospheric aerosols due to aerosols greater mass. HSRLs use narrow band laser and optical filters to get two independent signals. The schematic diagram of HSRL

is as follows: XXXVIII Meeting of the Italian Section of the Combustion Institute Figure 1. Schematic diagram of high spectral resolution lidar. As Figure 1 shows, seed injection-locked laser sends narrow-band beams with the wavelength of 1064nm and 532nm and a telescope receives the backscattering light by atmospheric molecules and aerosols. After the telescope, light is separated to two beams by a dichroic mirror. The IR beam with 1064nm wavelength is detected by a normal way and the HSRL technique is applied to 532 nm wavelength signal. The 532 nm backscatter signal is split between different channels corresponding to the parallel and orthogonal polarization of the backscattered light from aerosols and to the molecular signal. The molecular channel is used to retrieve the profile of extinction and all channels are used to retrieve profiles of aerosol backscatter coefficient and aerosol linear depolarization ratio. A frequency locking system is used to keep the receiver frequency locked with laser source with high accuracy. In order to evaluate the effect of system parameters and to obtain their optimal values, a system simulation has been done. The flow diagram of the system simulation process is as follows: Figure 2. The flow diagram of the system simulation process.

Figure 2 shows the system simulation consisting of four steps: modelling atmosphere, forward models, synthetic observations, inversion. The details are as follows: 1. The step of modelling atmosphere includes modelling of atmosphere and aerosol distribution. Here aerosol distribution modelling considers the three cases: clean sky, light pollution and heavy pollution. 2. In the e step of forward modelling molecular scattering Doppler broadening by thermal motion, aerosol scattering Doppler broadening by wind and the movement of the platform, and performance of HSR filter are evaluated. 3. In the third step, synthetic observations are considered by including the calculation of the received backscattering signals and SNR of molecular channel signal by HSRL in all the atmospheric conditions taken into consideration. The received molecular and aerosolic signals are as follows [3]: and r β exp 2 d (1) r β exp 2 d. (2) Here, r and r are the received signals, and contain all range-independent variables, r is the range from lidar to the scattering volume, O(r) is the laser-beam receiver-field-of-view overlap function, β and β are the atmospheric backscatter coefficients by molecules and aerosols at range r respectively. is the atmospheric extinction coefficient. 4. In the fourth step the inversion algorithm to retrieve aerosol optical properties, including aerosol extinction coefficient, backscattering coefficient, lidar ratio, etc are applied. The last step includes the calculation of the relative error on retrieved aerosol extinction and the aerosol extinction. These errors come from two aspects: one is aerosol to molecular channel crosstalk and the other is from the signal-to-noise ratio. When the minimum relative error of aerosol extinction is found, optimal system parameters are recorded. 3. Simulation results By inputting atmosphere molecular model, aerosol model and different system parameters, simulation results are obtained that are summarized in the following:

Figure 3. Frequency spectral of lidar backscattering signal. In Figure 3, it can be seen that the frequency distribution of the light backscattered from the atmosphere consists of a narrow spike near the frequency of the laser transmitter caused by particulate scattering (low velocity, small broadening effect) riding on a much broader distribution produced by molecular scattering. Figure 4. The received signals of aerosol and molecular channels. (a) Received signal in aerosol channel; (b) Received signal in molecular channel. Figure 4 shows that signals will be separated to two channels (Mie channel and molecular channel) after passing high spectral resolution etalon. Cross talks will occur in the two channels. The cross talk in molecular channel (i.e. the leak of part aerosol backscatter in it) in some circumstance could cause a significant distortion in the retrieval of the aerosol extinction coefficient. Simulation results also shows that the signal scattered by aerosol is strongly depended on the laser linewidth. So a laser with very narrow linewidth is necessary. After simulating the received signal with crosstalk and noise, aerosol extinction

coefficient can be obtained. By comparing the retrieved extinction coefficient with the input value, the relative errors of the extinction coefficient depend on the bandwidth of the high spectral resolution filter. Simulation results show that crosstalk is the main source of error when the filter bandwidth is small while noise becomes dominant when the filter bandwidth is big, so an optimal bandwidth can be found. For aerosols at different heights, the impacts of cross talk and noise on retrieved extinction coefficient are different. Simulation results show that high altitude cirrus exhibit a distortion in the retrieval of the aerosol extinction profile which is dominated by the cross talk effect. For elevated layers (as could be a Saharan dust layer), the distortion is dominated by noise. 4. Conclutions High spectral resolution lidars can measure aerosol vertical profile without assumptions of the aerosol extinction-to-backscatter ratio, offering both high vertical and temporal resolution. Through system simulation, the effects of system parameters and their optimal values have been found. Our simulation results also show that the accuracy of retrieved aerosol extinction coefficient is higher at low height than in high height range. References [1] Hair J. W. et al. Airborne High Spectral Resolution Lidar for profiling aerosol optical properties, Applied Optics, 6734-6753 (2008) [2] Hoffman D.S., Confocal Fabry-Perot Interferometer Based High Spectral Resolution Lidar, PhD Thesis, Montana State University, Bozeman, 6 (2012) [3] Weitkamp C., Lidar Range-Resolved Optical Remote Sensing of the Atmosphere, Springer, 2005, p. 147. doi: 10.4405/38proci2015.XI3