Spherical Beam Volume Holograms Recorded in Reflection Geometry for Diffuse Source Spectroscopy

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Spherical Beam Volume Holograms Recorded in Reflection Geometry for Diffuse Source Spectroscopy Sundeep Jolly A Proposal Presented to the Academic Faculty in Partial Fulfillment of the Requirements for the Degree of Bachelor of Science in Electrical Engineering with Research Option Author:... Sundeep Jolly Undergraduate Student School of Electrical and Computer Engineering School of Physics Certified by:... Dr. Ali Adibi Faculty Advisor Associate Professor School of Electrical and Computer Engineering Accepted by:... Dr. Douglass Williams Associate Chair for Undergraduate Affairs Professor School of Electrical and Computer Engineering School of Electrical and Computer Engineering College of Engineering Georgia Institute of Technology Atlanta, Georgia December 2006

Spherical Beam Volume Holograms Recorded in Reflection Geometry for Diffuse Source Spectroscopy Sundeep Jolly Faculty Advisor: Dr. Ali Adibi A Proposal Presented to the Academic Faculty in Partial Fulfillment of the Requirements for the Degree of Bachelor of Science in Electrical Engineering with Research Option School of Electrical and Computer Engineering College of Engineering Georgia Institute of Technology Atlanta, Georgia December 2006 ABSTRACT Recent developments in volume holographic materials, methods, and techniques have allowed for the development of novel data storage, optical processing, imaging, interferometric, and spectroscopic technologies [1-4, 6, 8]. Multimodal multiplex spectroscopy (MMS) has been demonstrated to increase the optical throughput of a spectrometer as opposed to that of conventional optical spectrometers [5] and has been implemented using three-dimensional photonic crystals [5] and spherical-beam volume holograms [6-7, 9] as spectral diversity filters. While such efforts have resulted in compact and sensitive Fourier-transform holographic spectrometers [8], there still remains much room for performance improvements. Previous studies [6,7,9] have proven the utility of spherical-beam volume holograms recorded in the transmission geometry as spectral diversity filters for spectrometers; however, limited work has been done with spherical-beam volume holograms recorded in the reflection geometry. It is the major goal of the current study to gauge the potential of reflection geometry holograms recorded on photopolymer film for compact, efficient, and sensitive spectrometers as compared to that of transmission geometry holograms. For a baseline comparison, studies of the spectral operating range and resolution of holograms for the spectroscopic application recorded in both geometries will be performed. Time permitting, studies of the efficacy of reflection geometry holograms in an implementation of a compact Fourier-transform holographic spectrometer will be performed.

Table of Contents 1 Introduction and Literature Review 4 2 Problem Statement 6 3 Research Goals 8 3.1 Low-Target Goals... 8 3.2 Ideal-Target Goals... 9 3.3 High-Target Goals... 9 3.4 Project Timetable... 10 4 Implications and Future Research 11 5 References 12

1 Introduction and Literature Review Recent developments in volume holographic materials, methods, and techniques have allowed for the development of novel data storage [1,4], optical processing [4], imaging [2,4], interferometric [4], and spectroscopic [8] technologies. Because of the demand for novel optical technologies employing holographic techniques (especially applications in data storage and integrated optical systems), there has been a recent surge of research activity in the area. It is of notice that holographic technologies are already replacing more conventional optical technologies in applications such as data storage and spectroscopy. Highly sensitive and portable spectrometers are desirable for applications in biological and environmental sensing especially because the optical sources of interest are diffuse in nature. Conventional spectrometers generally operate by employing gratings for wavelength dispersion and demultiplexing. The intermediate signal achieved by the grating is then usually retrieved by a photodetector for data collection. Because the overlap of multiple spatial modes in some incident signals (for instance, as occurs with diffuse sources) can result in false output patterns, spatial filtering is necessary and is accomplished in conventional spectrometers by means of a slit-lens collimating setup. Although spatial filtering in such a manner can effectively increase the resolution which can be achieved with a grating-based conventional spectrometer, the slit-lens collimator blocks most of the intensity of the original light source [5]. Because of the resolution-throughput tradeoff caused by spatial filtering, conventional spectrometers are highly limited when used with diffuse, incoherent light sources, such as those often encountered in biological and environmental sensing applications. Multimodal multiplex spectroscopy (MMS) has been developed as a method of spectroscopy particularly useful when dealing with diffuse sources [5]. In MMS, an input light source is projected 4

onto a spectral diversity filter (SDF), which converts the input spatial-spectral signal into an output spectral diversity pattern. In this way, the SDF acts analogously to a more general wavelength dispersive element (such as a prism or holographic grating) but is readily more flexible and eliminates the resolution-efficiency tradeoff of conventional spectrometers. An MMS system would employ a Fourier-transforming lens and a charge-coupled device for processing and capturing of the intermediate signal achieved by the SDF. Post-processing of the output signal retrieved by the CCD can successfully estimate the spectrum of the input signal [5]. To date, SDFs have been implemented using three-dimensional photonic crystals [5] and spherical-beam volume holograms (SBVHs) [6,7]; MMS systems based on both of these two SDF implementations have been proposed, prototyped, and studied for sensitivity [5,8,9]. Recently, MMS systems for laboratory settings have entered the marketplace, demonstrating the capabilities and promise of this new technology. Of high interest, however, are compact and inexpensive spectrometers employing spherical-beam volume holograms as SDFs for their low cost and high robustness as compared to conventional optical spectrometers. Incident Beam Diffracted Crescent Fourier-Transforming Lens CCD Imager Hologram To PC Interface Fig. 1. Configuration for the holographic spectrometer. The diffracted crescent from the hologram is retrieved by the CCD for post-processing and spectrum retrieval. Currently, volume holographic Fourier-transform spectrometers consisting of one of more volume holograms recorded in a piece of photopolymer along with a Fourier-transforming lens and a detector array have been demonstrated [8]. A typical slitless holographic spectrometer configuration is portrayed in Fig. 1. The key operating feature of the holographic spectrometer is the retrieval of the intermediate spatial-spectral signal achieved by the holographic spectral diversity filter (i.e., the diffracted crescent) by the detector array. 5

2 Problem Statement Optimizing the parameters that define the spectral diversity filter is essential to improving the sensitivity and resolution of holographic spectrometers. Spherical-beam volume holograms have been shown to be usable for spectral diversity filtering [6] and a compact Fourier-transform spectrometer has been demonstrated using a SBVH as the SDF [8]. Plane Wave \ L Point Source θ 1 θ 2 d (a) L Plane Wave Point Source θ 1 θ 2 d (b) Fig. 2. Recording geometries for spherical beam volume holograms. In the transmission geometry (a), the plane wave and the spherical beam enter the hologram from the front face. In the reflection geometry, the plane wave and the spherical beam enter the hologram from opposing sides. 6

Recording geometries for spherical beam volume holograms are shown in Fig. 2. The recording of a SBVH involves the interference of a plane wave (i.e., the signal beam) and a spherical beam (i.e., the reference beam) in the plane of the photopolymer being used. In the transmission geometry, the plane wave enters the photopolymer from the same direction as the spherical beam. In the reflection geometry, the plane wave and the spherical beam enter the photopolymer from opposing directions. Both recording geometries offer unique transmission and diffraction characteristics for recorded holograms. Previous studies have determined the efficacy of SBVHs recorded in the transmission geometry as SDFs [6,9]. A preliminary study has indicated the potential of SBVHs recorded in the reflection geometry as SDFs and for implementation in compact Fourier-transform spectrometers [7]. However, while the potential of reflection geometry SBVHs for spectral diversity filtering has been asserted, studies of the performance of reflection geometry holograms in spectral diversity filtering and as the key element for a compact holographic spectrometer have not been conducted. It is the major goal of the current study to gauge the potential of reflection geometry holograms recorded on photopolymer film for compact and highly sensitive spectrometers as compared to that of transmission geometry holograms. For a baseline comparison, studies of the spectral operating range and output holograms recorded in both geometries will be performed. Time permitting, studies of the efficacy of reflection geometry holograms in an implementation of a compact, Fourier-transform spectrometer will be performed. 7

3 Research Goals In order to characterize the performance of spherical beam volume holograms recorded in reflection geometry as spectral diversity filters in a holographic spectrometer, several criteria will be examined. The examination of such criteria will be accomplished through a reading setup mimicking the configuration for the holographic spectrometer given in Fig. 1. 3.1 Low-Target Goals The spectral operating range for a given spectrometer is an important parameter which defines the range of incident wavelengths for which the spectrometer is able to perform most accurately. More specifically, the spectral operating range defines the range of incident wavelengths for which the spectrometer is most sensitive and offers the best resolution and hence the best performance. As a primary goal, the spectral operating range for holographic SDFs recorded in both the transmission geometry and the reflection geometry will be characterized. Similar recording parameters (i.e., recording time, angle between signal and reference beams, recording beam intensities) will be used to record holograms in both geometries on separate pieces of photopolymer. A monochromator will be used to provide the incident light source. By varying the incident wavelength of the incident source, the spectral operating range for the holograms can be characterized. 3.2 Ideal-Target Goals Sensitivity, resolution, and the signal-to-noise-ratio are important for characterization of the total performance of a holographic spectrometer. Measurements of sensitivity and resolution will be accomplished by using a reading setup in conjunction with a monochromator for wavelength tunablility of the input source. The resolution can be 8

directly determined from the relationship between a change in incident wavelength and the structure of the output pattern retrieved by the CCD imager. The sensitivity can be determined by quantifying the quality of the output pattern retrieved by the CCD and relating such a quantity to the incident wavelength. The signal-to-noise-ratio can be determined by directly comparing the quality of the output pattern retrieved by the CCD to the incident light intensity on the face of the hologram and using signal-processing tools to determine the amount of noise contained within the output. Since it is expected that the measurements for the above quantities will not be without error (for, at least, the first few measurements taken), appropriate corrections will be taken to perfect the measurement schemes for these quantities. It is expected that the development of proper measurement techniques for the quantities above will take several weeks. 3.3 High-Target Goals The application of the holographic spectrometers for diffuse source spectroscopy is of particular interest. Using a diffuser along with an incident wavelength-tunable light source (i.e., a monochromator), studies of all the parameters discussed before (spectral operating range, sensitivity, resolution, and signal-to-noise-ratio) will be performed for holograms recorded in both geometries to determine the performance of these holograms under diffuse incident source conditions. Multiplexing in volume holograms has been shown [4] to allow for increased performance for holographic spectrometers utilizing holograms recorded in the transmission geometry. Multiplexing involves the recording of multiple holograms in a single piece of photopolymer which, in the case of the holographic spectrometers, allows for greater output resolution while retaining the same photon throughput (and therefore not damaging the efficiency of the holograms). As a high-target goal, studies to determine the ideal multiplexing scheme for holograms recorded in the reflection geometry will be performed and will allow for a comparison of the performance of multiplexed holograms recorded in reflection geometry and that of multiplexed holograms recorded in transmission geometry. 9

3.4 Project Timetable January 2007 February 2007 March 2007 April 2007 May 2007 August 2007 September 2007 October 2007 November 2007 December 2007 background reading, create recording / reading setup finalize recording / reading setups, record holograms, preliminary analysis of hologram characteristics (e.g., diffraction efficiency) record holograms, analyze spectral diversity characteristics roughly, characterize spectral operating range for all holograms begin measurements of sensitivity, resolution, and signal-to-noiseratio for holograms work on measurements of sensitivity, resolution, and signal-tonoise-ratio for holograms complete measurements for sensitivity, resolution, and signal-tonoise-ratio begin writing of final thesis, begin measurements for diffuse sources, look into multiplexing methods thesis writing, high-target goals thesis writing, high-target goals complete thesis and thesis presentation Note that this timetable will be developed into a more formal Gannt Chart detailing a breakdown of tasks before work on the project begins. This timetable will be modified and update to suit the dynamic, developing needs of the project. 10

4 Implications and Future Research It is the goal of this research to produce the parameters which will eventually lead to a viable, robust, and versatile volume holographic spectral diversity filter for inclusion as part of a commercially-viable, compact, efficient, and inexpensive MMS-based holographic spectrometer. Such spectrometers have tremendous applications when dealing with diffuse input light sources and where portability and robustness in a spectrometer is highly desirable. The successful implementation of a spectral diversity filter using a spherical beam volume hologram recorded in the reflection geometry would invariably be followed up by studies to improve the efficacy of such an SDF by further investigation into, for instance, multiplexing methods for overcoming the resolution tradeoff that occurs when using photopolymers of varying thicknesses for better throughput. 11

5 References 1. D. Brady and D. Psaltis, Control of Volume Holograms, Journal of Optical Society of America A 9, 1167 (1992) 2. A. Sinha, G. Barbastathis, W. Liu, and D. Psaltis, Imaging using volume holograms, Optical Engineering 43(9), 1959 (2004) 3. Y. Yang, A. Adibi, and D. Psaltis, Comparison of transmission and the 90-degree holographic recording geometry, Applied Optics 42, 3418 (2003) 4. G. Barbastahis and D. Psaltis, Volume holographic multiplexing methods, Holographic Data Storage, Eds: H. Coufal, D. Psaltis, and G. Sincerbox. Springer, New York, 2000. 21-59. 5. Z. Xu, Z. Wang, M. Sullivan, D. Brady, S. Foulger, and A. Adibi, Multimodal multiplex spectroscopy using photonic crystals, Optics Express 11, 2126 (2003) 6. A. Karbaschi, C. Hsieh, O. Momtahan, A. Adibi, M. Sullivan, and D. Brady, Qualitative demonstration of spectral diversity filtering using spherical beam volume holograms, Optics Express 12, 3018 (2004) 7. C. Hsieh, O. Momtahan, A. Karbaschi, A. Adibi, M. Sullivan, and D. Brady, Role of recording geometry in the performance of spectral diversity filters with spherical beam volume holograms, Optics Letters 30, 2, 186 (2005) 8. C. Hsieh, O. Momtahan, A. Karbaschi, and A. Adibi, Compact Fourier-transform volume holographic spectrometer for diffuse source spectroscopy, Optics Letters 30, 8, 836 (2005) 9. O. Momtahan, C. Hsieh, A. Karbaschi, A. Adibi, M. Sullivan, and D. Brady, Spherical beam volume holograms for spectroscopic applications: modeling and implementation, Applied Optics 43, 6557 (2004) 12

10. O. Momtahan, C. Hsieh, A. Adibi, and D. Brady, Analysis of slitless holographic spectrometers implemented by spherical beam volume holograms, Applied Optics 45, 2955 (2006) 13