Canadian Centre for Climate Modelling and Analysis. CCCma AGCM4



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Canadian Centre for Climate Modelling and Analysis CCCma AGCM4 Knut von Salzen 1, Norman McFarlane 1, Jiangnan Li 1, Cathy Reader 1 Glen Lesins 2, Ulrike Lohmann 2, Betty Carlin 2 1 MSC, CCCma, Victoria, British Columbia, Canada 2 Dalhousie University, Halifax, Nova Scotia, Canada Presented at AEROCOM Workshop, Paris, June 2-3, 2003

CCCma AGCM4: Basic Features Spectral model (current resolution is T47) 35 vertical levels Hybrid moisture and chemical tracer variables for advection and horizontal diffusion Prognostic cloud microphysics (Lohmann and Roeckner 1996) Deep convection (Zhang and McFarlane 1995) Shallow convection (von Salzen and McFarlane 2002)

CCCma AGCM4: Basic Features (cont d) Fully coupled cycles of sulphur, mineral dust, and sea salt (black and organic carbon aerosol to come soon) Nine aerosol log-normal modes Correlated k-distribution method for gaseous transmission (Li and Barker 2002) Aerosol and cloud optical depth for 9 IR and 4 solar bands Subgrid-scale variability of cloud optical properties (Barker 1996) CLASS land surface scheme (Verseghy et al. 1992)

Aerosol and Precursors in GCM4: Emissions Species Surface Source Strength (Tg/Year) Reference DMS (gas) marine biosphere 17.3 Kettle et al. (1996) terrestrial biosphere 0.9 Spiro et al. (1992) SO 2 (gas) non-eruptive volcanoes 8.0 Spiro et al. (1992), Graf et al. (1997) biomass burning 2.5 Hao et al. (1990) fossil fuel use 66.8 Benkovitz et al. (1994) SO 4 = - - von Salzen et al. Black Carbon 1 anthropogenic 6.1 Liousse et al. (1996) biomass burning 5.6 Liousse et al. (1996) Organic Carbon 1 natural anthropogenic 16.2 29.6 Guenther et al. (1995) Liousse et al. (1996) biomass burning 59.3 Liousse et al. (1996) Sea Salt 2 natural - von Salzen et al. Mineral Dust 2 natural - Reader et al. 1 hydrophobic and hydrophilic components 2 accumulation and coarse modes

Sulphur Cycle in CCCma AGCM4 (JJA ugs/m 2 /day) HNO 3 = NH = 3 = CO 2 227 SO 4 O 3 H 2 O 2 SO 4 33 78 OH NO 3 (night) SO 4 HNO 3 O 3 H 2 O 2 16/12 CO 2 160 SO 2 OH (day) 32/2 NH 3 DMS Land Ocean

Parameterization of Convection: Basic Equations Entrainment Chemical/Microphysical Sources and Sinks Chemical/Microphysical Flux DivergenceEntrainment Detrainment Sources and Sinks Impuls Flux Divergence -for cloud water Detrainment - for gas and aerosol -otherwise Rainout and Washout Oxidation of S(IV)

Parameterization of Microphysical Processes in Stratiform Clouds Lohmann and Roeckner (1996): cloud droplet number concentration

Status of AEROCOM Runs Latest model run completed on May 17, 2003 with AEROCOM output variables Diagnostics currently being done AEROCOM output fields ready for download by end of June, 2003 Climate mode only (no nudging)

PS 2D Surface pressure Basic results on pressure levels -------------------------------- T 3D Temperature K U 3D Zonal wind M/S V 3D Meridional wind M/S Basic results on hybrid levels -------------------------------- GST 3D Temperature K GSU 3D Zonal wind M/S GSV 3D Meridional wind M/S RHC 3D Relative humidity % Mixing ratios on pressure levels -------------------------------- BCO 3D Black carbon (hydrophobic) mixing ratio BCY 3D Black carbon (hydrophilic) mixing ratio DMS 3D DMS mixing ratio kg-s/kg DUA 3D Min. dust acc. mode mixing ratio kg/kg DUC 3D Min. dust coarse mode mixing ratio kg/kg OCO 3D Organic carbon (hydrophobic) mixing ratio OCY 3D Organic carbon (hydrophilic) mixing ratio SSA 3D Sea salt acc. mode mixing ratio kg-nacl/kg SSC 3D Sea salt coarse mode mixing ratio kg-nacl/kg SO2 3D Sulphur dioxide mixing ratio kg-s/kg SO4 3D Sulphate mixing ratio kg-s/kg

Mixing ratios on hybrid levels ------------------------------ GBCO 3D Black carbon (hydrophobic) mixing ratio GBCY 3D Black carbon (hydrophylic) mixing ratio GDMS 3D DMS mixing ratio kg-s/kg GDUA 3D Min. dust acc. mode mixing ratio kg/kg GDUC 3D Min. dust coarse mode mixing ratio kg/kg GOCO 3D Organic carbon (hydrophobic) mixing ratio GOCY 3D Organic carbon (hydrophylic) mixing ratio GSSA 3D Sea salt acc. mode mixing ratio kg-nacl/kg GSSC 3D Sea salt coarse mode mixing ratio kg-nacl/kg GSO2 3D Sulphur dioxide mixing ratio kg-s/kg GSO4 3D Sulphate mixing ratio kg-s/kg Vertical integrals ------------------ VI01 2D Cloud liquid water path kg/m**2 VI02 2D Cloud ice water path kg/m**2 VI05 2D Black carbon (hydrophobic) burden VI06 2D Black carbon (hydrophylic) burden VI07 2D Organic carbon (hydrophobic) burden VI08 2D Organic carbon (hydrophylic) burden VI09 2D Sea salt acc. mode burden kg-nacl/m**2 VI10 2D Sea salt coarse mode burden kg-nacl/m**2 VI11 2D Min. dust acc. mode burden VI12 2D Min. dust coarse mode burden VI13 2D DMS burden kg-s/m**2 VI14 2D Sulphur dioxide burden kg-s/m**2 VI15 2D Sulphate burden kg-s/m**2 VI16 2D Hydrogen peroxide burden kg-s/m**2 VI17 2D Total water path kg/m**2

AB11 2D Aerosol absorption for sulphate aerosol in band 1 AB21 2D Aerosol absorption for sulphate aerosol in band 2 AB31 2D Aerosol absorption for sulphate aerosol in band 3 AB41 2D Aerosol absorption for sulphate aerosol in band 4 AB12 2D Aerosol absorption for sea salt aerosol in band 1 AB22 2D Aerosol absorption for sea salt aerosol in band 2 AB32 2D Aerosol absorption for sea salt aerosol in band 3 AB42 2D Aerosol absorption for sea salt aerosol in band 4 AB13 2D Aerosol absorption for mineral dust in band 1 AB23 2D Aerosol absorption for mineral dust in band 2 AB33 2D Aerosol absorption for mineral dust in band 3 AB43 2D Aerosol absorption for mineral dust in band 4 AB1T 2D Aerosol absorption for total aerosol in band 1 AB2T 2D Aerosol absorption for total aerosol in band 2 AB3T 2D Aerosol absorption for total aerosol in band 3 AB4T 2D Aerosol absorption for total aerosol in band 4 AO11 2D Aerosol optical depth for sulphate aerosol in band 1 AO21 2D Aerosol optical depth for sulphate aerosol in band 2 AO31 2D Aerosol optical depth for sulphate aerosol in band 3 AO41 2D Aerosol optical depth for sulphate aerosol in band 4 AO12 2D Aerosol optical depth for sea salt aerosol in band 1 AO22 2D Aerosol optical depth for sea salt aerosol in band 2 AO32 2D Aerosol optical depth for sea salt aerosol in band 3 AO42 2D Aerosol optical depth for sea salt aerosol in band 4 AO13 2D Aerosol optical depth for mineral dust in band 1 AO23 2D Aerosol optical depth for mineral dust in band 2 AO33 2D Aerosol optical depth for mineral dust in band 3 AO43 2D Aerosol optical depth for mineral dust in band 4 AO1T 2D Aerosol optical depth for total aerosol in band 1 AO2T 2D Aerosol optical depth for total aerosol in band 2 AO3T 2D Aerosol optical depth for total aerosol in band 3 AO4T 2D Aerosol optical depth for total aerosol in band 4 W1A 2D Aerosol water sulphate W2A 2D Aerosol water sea salt acc. mode W2C 2D Aerosol water sea salt coarse mode WACT 2D Aerosol water sulphate + sea salt

Emissions --------- BCOE 2D Black carbon (hydrophobic) emissions BCYE 2D Black carbon (hydrophylic) emissions DAFX 2D Min. dust acc. mode emissions DCFX 2D Min. dust acc. mode emissions OCOE 2D Organic carbon (hydrophobic) emissions OCYE 2D Organic carbon (hydrophylic) emissions Dry deposition -------------- DDBC 2D Black carbon (hydrophobic) dry deposition DDBY 2D Black carbon (hydrophylic) dry deposition DDDA 2D Min. dust acc. mode dry deposition DDDC 2D Min. dust coarse mode dry deposition DDNA 2D Sea salt acc. mode dry deposition kg-nacl/m**2/sec DDNC 2D Sea salt coarse mode dry deposition kg-nacl/m**2/sec DDOC 2D Organic carbon (hydrophobic) dry deposition DDOY 2D Organic carbon (hydrophylic) dry deposition DD6 2D Sulphate dry deposition kg-s/m**2/sec Wet deposition -------------- WDBC 2D Black carbon wet deposition WDMA 2D Min. dust acc. mode wet deposition (total) WDMC 2D Min. dust coarse mode wet deposition (total) WDNA 2D Sea salt acc. mode wet deposition kg-nacl/m**2/sec WDNC 2D Sea salt coarse mode wet deposition kg-nacl/m**2/sec WDOC 2D Organic carbon wet deposition WDD6 2D Sulphate wet deposition due to deep convection kg-s/m**2/sec WDL6 2D Sulphate wet deposition due to stratiform clouds kg-s/m**2/sec WDS6 2D Sulphate wet deposition due to shallow convection kg-s/m**2/sec

Chemical sources and sinks -------------------------- ---------------- DOX4 2D Suphate production in gas-phase kg-s/m**2/sec SDHP 2D Sulphate production in deep convection due to hydrogen peroxide kg-s/m**2/sec SDO3 2D Sulphate production in deep convection due to ozone kg-s/m**2/sec SLHP 2D Sulphate production in stratiform clouds due to hydrogen peroxide kg-s/m**2/sec SLO3 2D Sulphate production in stratiform clouds due to ozone kg-s/m**2/sec SSHP 2D Sulphate production in shallow convection due to hydrogen peroxide kg-s/m**2/sec SSO3 2D Sulphate production in shallow convection due to ozone kg-s/m**2/sec Extra ----- RHOA 3D Air density on hybrid levels kg/m**3