Di-PPG-2 Myreth-10 Adipate



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DS-154R-3 October 15, 2002 INCI Name: Di-PPG-2 Myreth-10 Adipate * is an 100% active alkoxylated di-ester of Myristyl Alcohol and Adipic Acid and represents novel chemistry as one of an entirely new class of emollients from Croda. As an emollient, offers unique benefits in that it is both hydroactive and surfactant-friendly, as well as mild, making it ideal for products like body washes, liquid soaps, facial cleansers and shampoos, particularly baby shampoos. Benefits Water Dispersible Surfactant Silky Emollience Detangler/Slip Enhancer Improved Wet Combing Suitable for Clear Systems Solubilizes Benzophenone-3 Approved for Use in Europe acquires its unique properties from its bulk and stereochemistry as an alkoxylated di-ester of ethoxylated propoxylated Myristyl Alcohol and Adipic Acid. CH 3 CH 3 (CH 2 ) 13 O(CH 2 CHO) 2 (CH 2 CH 2 O) 10 O C CH 3 CH 3 (CH 2 ) 13 O(CH 2 CHO) 2 (CH 2 CH 2 O) 10 C O * is covered under U.S. Patent US #5,302,377 and it use in Personal Care is covered under US Patent #5,455,025. Croda Inc 300 Columbus Circle, Edison, NJ 08837 Tel 732-417-0800 Fax 732-417-0804 Website www.crodausa.com Sederma Inc. Tel 732-692-1652 Fax 732-417-0804 Croda Inc Midwest Sales Office 1520 West Ardmore Avenue Itasca IL 60143-1109 Tel 1-888-44CRODA Fax 630-467-0424 Croda Inc West Coast Sales Office 385 S Acacia Avenue Fullerton CA 92831-4748 Tel 714-526-1162 Fax 714-526- 0637 Croda Miami Inc 200 South Park Road, Suite, 303, Hollywood, FL. 33021 Tel 1-888-84CRODA Fax 954-989-8186 Sol Kaplan & Son PO Box 240234 Memphis TN 38124-0234 Tel 901-685-0323 Fax 901-763-3612 Croda Canada Ltd 221A Racco Parkway, Vaughan, Ontario L4J8X9 CANADA Tel 905-886-1383 Fax 905-886-4753 Non-Warranty: All information contained herein is intended primarily to demonstrate the utility of Croda products. We assume no liability in the presentation of this data, nor should this information be construed as granting license to practice any methods or compositions of matter covered by U.S. or foreign patents.

Performance Data Skin Care: In a blind performance test, panelists were asked to evaluate a body wash (see formula below) for product feel during lathering and for afterfeel on drying. The overwhelming preference in both wet and dry feel was the body wash containing which was preferred by nearly 75% of panel members, compared to a prototype using a comparable emollient. Body Wash Panel Evaluation vs. PEG-6 Capric/Caprylic Glycerides 15 Panel Preference 10 5 Wet Feel Dry Feel 0 X Y NP X=Sample with PEG-6 Capric/Caprylic Glycerides Y=Sample with NP=No Preference Body Wash Formula (BP-53) % w/w Ingredients X Y PART A Deionized Water 54.00 54.00 SLES, 3 mole 20.00 20.00 CROSULTAINE C-50 (Cocodimonium Hydroxysultaine) 12.00 12.00 Disodium EDTA 0.10 0.10 PART B INCROMIDE CA (Cocamide DEA) 3.00 3.00 GLYCEROX 767 (PEG -6 Capric/Caprylic Glycerides) 3.00 (Di-PPG-2 Myreth-10 Adipate) 3.00 CROTHIX LIQUID (PEG-150 Pentaerythrityl Tetrastearate (and) PEG-6 Caprylic/Capric Triglyceride (and) Water) 3.00 3.00 PART C CROTEIN C-50 (Hydrolyzed Collagen) 1.00 1.00 INCROMECTANT LAMEA (Acetamide MEA (and) Lactamide MEA) 1.00 1.00 CITRIC ACID 1.00 1.00 GERMABEN 11 (Methyl Paraben (and) Butyl Paraben (and) Ethyl Parab en (and) Propyl Paraben) 1.00 1.00 PROCEDURE: Combine Part A ingredients and mix until clear. Combine Part B ingredients and heat to 50ºC, mixing until clear. Slowly add Part B to Part A, mixing well. Add Part C ingredients individually and mix until uniform. ph = 4.58; Viscosity=1,100 cps (RVT Spindle #4 @ 10rpm, RT) 2

Hair Care: In a separate study was found superior in reducing the wet combing forces of virgin hair tresses, as shown by the graph below. The combing work and peak force of tresses treated with a shampoo containing CROMOLLIENT SCE were evaluated against those treated with a shampoo containing Polyquaternium-10. Values given are percent reductions as compared to a control. The improvements in wet coming for tresses are dramatic, as seen by the 50+% decrease in peak combing force. Given this, can be of immense benefit in the formulation of baby shampoos, as it gives formulators an ideal means of keeping baby's fine hair more snarl-free. Reduction in Wet Combing Forces vs. Polyquaternium-10 % Reduction 80 60 40 20 0-20 Polyquaternium-10 Peak Load Total Work Control represented by the baseline Applications provides a substantial improvement in the wet combing properties of virgin hair. Body Washes Liquids Soaps Facial Cleansers Baby Shampoos 2-in-1 and Conventional Shampoos Bath Oils After Shave Products Low VOC Products Pre-Solubilizer for Benzophenone- 3 and for hair dye actives is suitable for a wide range of products and confers a silky emollience that is distinct and immediately perceptible. Our applications work indicates that the di-ester works especially well in clear surfactant systems (i.e., body washes) and appears to have little effect on foaming when used at up to 3% active. Additional testing has shown is an excellent wax solvent for lipsticks or lip balms (see formula SC-305, page 5). also possesses extremely effective solubilizing properties so much so, that even very difficult materials like the sunscreen Benzophenone-3 can be presolubilized at 3

concentration levels up to as high as 20-25. The di-ester can also be used as a presolubilizer for hair dyes or as a pigment wetting agent for Mica or TiO2. Use level: 1-5% for surfactant-based systems; 1-25% for other applications. Mineral Oil Almond Oil Alcohol SD40 Solubilities CRODAMOL PMP (PPG-Myristyl Ether Propionate) INCRODET TD-7 C (Trideceth-7 Carboxylic Acid) ALS TEALS SLES (3 mol) Water:Alcohol: 75:25 Insoluble 50:50 25:75 Deionized Water (ph 9.0) Glycerin Propylene Glycol Dispersible Insoluble Dispersible Typical Analysis APPEARANCE Clear liquid COLOR (APHA) < 20 ODOR Mild, characteristic ACID VALUE < 1.0 SAPONIFICATION VALUE 70 ph 6.0 4

Lip Balm with Benzophenone-3 SC-305 This lip balm formula highlights and demonstrates the diester s use as a wax solvent and its compatibility with common lipstick ingredients. The use of here results in a hard, stable stick that has a fine crystal structure and no observable syneresis. also helps to solubilize the sunscreen Benzophenone-3. Ingredients % PART A SYNCROWAX HGL-C (C18-36 Acid Triglyceride) 12.0 SYNCROWAX ERL-C (C18-36 Acid Glycol Ester) 3.0 Petrolatum 61.7 SUPER STEROL ESTER (C10-30 Cholesterol/Lanosterol Esters) 3.0 PART B (Di-PPG-2 Myreth-10 Adipate) 10.0 Benzophenone-3 5.0 Ethylhexyl Dimethyl PABA (1) 5.0 PART C Methyl Paraben 0.1 Propyl Paraben 0.2 PROCEDURE Combine ingredients of Part A and heat to 80-85 C, mixing until homogenous. Cool to 75 C. Combine ingredients of Part B with mixing and heat to 75 C. Add Part B to Part A with mixing. Then add Part C ingredients individually, mixing well. Cool mixture to 70 C and pour into molds. 1) Escalol 507 (ISP/Van Dyke) September 13, 2000 5

After-Shave Lotion: High Alcoholic Type BP-54 This after shave lotion contains a high alcohol content and demonstrates the excellent solubilizing properties of. Ingredients % PART A Deionized Water 13.80 PHYTOTAL AI (Glycerin (and) Butylene Glycol (and) Euphrasia Officinalis Extract (and) Magnolia Biondii Flower Extract (and) Melissa Officinalis (Balm Mint) Leaf Extract (and) Lecithin) 3.00 KAVA KAVA (PEG-8 (and) Water (and) Piper Methysticum Extract (and) PEG-8/SMDI Copolymer) 2.00 Butylene Glycol 1.00 PART B SD Alcohol 40 75.00 (Di-PPG-2 Myreth-10 Adipate) 5.00 Fragrance 0.20 ph=7.3 ±0.5 PROCEDURE: Combine ingredients of Part A with mixing. Combine ingredients of Part B, mixing well, and add to Part A. Mix thoroughly before filling. September 13, 2000 6

Soothing After-Shave Lotion BP-55 This after-shave lotion confers a lubricious skin feel due to the use of as an emollient in the formula. KAVA KAVA and PHYTOTAL AI provide soothing effects that help alleviate the stinging sensation often felt after shaving. Ingredients % PART A Deionized Water 82.70 Carbomer 934 (1) 0.20 Xanthan Gum 0.10 Disodium EDTA 0.05 PART B (Di-PPG-2 Myreth-10 Adipate) 3.00 CRODACOL CS-50 (Cetearyl Alcohol) 1.25 POLAWAX (Emulsifying Wax NF) 2.00 DISTRESSINE (Petrolatum (and) Butyrospermum Parkii (and) Pisces (and) Laureth-3 (and) Tocopheryl Acetate (and) Zea Mays 0.25 PART C (Di-PPG-2 Myreth-10 Adipate) 0.25 Dimethicone (2) 0.50 PART D Deionized Water 2.00 Triethanolamine 0.20 KAVA KAVA (PEG-8 (and) Water (and) Piper Methysticum Extract (and) PEG-8/SMDI Copolymer) 2.00 PHYTOTAL AI (Glycerin (and) Butylene Glycol (and) Euphrasia Officinalis Extract (and) Magnolia Biondii Flower Extract (and) Melissa Officinalis (Balm Mint) Leaf Extract (and) Lecithin) 2.00 Aloe Vera Gel (3) 1.50 Pentylene Glycol (4) 2.00 PROCEDURE Disperse carbomer of Part A in water with rapid agitation, then xanthan gum. Add remaining ingredient of Part A and heat to 70-75 C. Combine ingredients of Part B and heat to 70-75 C. Add Part B to Part A with mixing and begin cooling. Combine Part C ingredients and add to Part A/B mixture when temperature reaches 50 C. Add Part D ingredients when mixture has cooled to 40 C. 1) Carbopol 934 (B.F. Goodrich) 2) Silicone HL-88 (Barnet Products Corp.) September 13, 2000 3) Whloe Leaf Aloe Vera Gel (Coats Aloe International) 4) Hydrolite 5 (Dragoco) 7

Low VOC Hair Spray HP-213 The compatibility of in hydroalcoholic systems makes it an ideal emollient for this low VOC hairspray. Ingredients % SD Alcohol 40 53.80 Isobutylene/Ethylmaleimide/Hydroxyethylmaleimide Copolymer (1) 6.00 (Di-PPG-2 Myreth-10 Adipate) 3.00 Deionized Water 37.20 PROCEDURE Disperse resin in alcohol, with mixing. When mixture is clear, add remaining two ingredients one at a time, mixing well after each. 1) Aquaflex FX-64 (ISP) September 13, 2000 8