ADHESIVE BONDING PERFORMANCE OF GA COATED 590 MPa TENSILE STRENGTH STEELS



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ADHESIVE BONDING PERFORMANCE OF GA COATED 590 MPa TENSILE STRENGTH STEELS Susan Wolf ArcelorMittal Global R&D East Chicago

Acknowledgements Chann Cheng, Benda Yan, Jayanth Chintamani, ArcelorMittal Global R & D East Chicago Mike Golden & Jagdeesh Bandekar Dow Automotive

Outline Background Test Materials GA coated materials Adhesives Residual Stress Measured by XRD Cracks in Coating Test Method Results Conclusions

Background Light weighting in the automotive industry is a constant objective that is increasingly obtained using: Advanced high strength steels (AHSS) Crash resistant and fracture toughened adhesives In crash sensitive applications, adhesives are generally avoided on galvanneal (GA) coated steels. GA coated 780 MPa AHSS were shown to have cohesive failure and good bond strength. The subject study focused on the adhesive bonding performance of GA 590 MPa materials bonded with adhesives of different moduli of elasticity. GA coated IF EDDS steels were included for comparison.

Test Materials GA coated test materials include 590Y (dual phase) 0.7 & 1.6 mm 590R (high yield to tensile ratio) 1.2, 1.5, 1.7 mm 590T (TRIP) 1.5 mm 270E (IF EDDS) 0.7 & 1.5 mm Test materials were bonded with up to three adhesives. BETAMATE TM 1488, crash resistant structural, modulus 1400 MPa. BETAMATE TM 1022DUS, fracture toughened structural, modulus 2000 MPa. BETAMATE TM 73305GB, structural, hem flanging, modulus 4100 MPa.

Test Materials Material Code Gauge (mm) Coating Wt (g/m²) % Fe Fe Content (g/m²) Width of GA removed by tape in 60 o V- Bend Test (mm) Residual Stress (MPa) 590Y-C 0.7 37.5 10.5 3.9 2-26 590Y-96 1.6 53.7 12.6 6.8 9-35 590Y-97 1.6 51.3 12.4 6.4 3-53 590R-61 1.2 40.1 10.8 4.3 2-85 590R-98 1.5 39.2 11.6 4.5 3-64 590R-12 1.5 38.9 9.7 3.8 3-82 590R-53 1.7 38.8 11.3 4.4 3-58 590T-05 1.5 53.1 11.7 6.2 5-50 590T-897 1.5 43.6 12.1 5.3 8-82 270E-35 0.7 47.1 10.8 5.1 3-3 270E-19 1.5 39.2 12.1 4.7 3-50 270D-06 1.5 37.3 10.8 4.0 3-33

Residual Stress Measured by XRD Opposite stresses are felt on both sides of the interface; i.e. compressive stress on substrate leads to a tension stress on the coating. Results show that there is a moderate to high compressive stress on the steel surface for all materials, except the thin gauge EDDS. Typically, a larger lattice mismatch exists between IF EDDS and the Γ phase in the GA, which may cause breakage of the lattice bonding at the interface to release the residual stress.

Residual Stress Cracks in Coating EDDS 590Y 590R 590T EDDS

Lap Shear Test Method The 25 x 102 mm samples were solvent wiped before bonding. o 12 test materials were bonded with BETAMATE TM 1488. o 6 test materials were bonded with BETAMATE TM 1022DUS & BETAMATE TM 73305GB. In some cases, backing plates of 1.6 mm sheet steel were bonded to the back of each specimen. The average joint had an overlap of 12.7 mm and a bond thickness of 0.25 mm controlled by glass beads. The adhesive was cured for 20 minutes at 170 C. Specimens were pulled on an Instron tensile test machine at 50 mm/minute at room temperature. The shear strength in MPa and the failure mode as % cohesive failure were reported.

Evaluation of failure mode Lap Shear Test Method OK Cohesive Failure (CF) = failure in the adhesive Avoid May be OK if bond strength is good. Not OK Coating Delamination Adhesive Failure = failure of adhesive to substrate

Shear Strength (MPa) Results DOW BETAMATE 1488 Lap Shear Strength (MPa) of Test Materials Bonded with BM1488 40 35 30 25 20 15 10 5 Backing Plate 0 No Backing Plate 590Y C 590Y 96 590Y 97 590R 61 590R 98 590R 12 590R 53 590T 05 590T 897 270E 35 270E 19 270D 06 590 MPa Materials EDDS IF Materials

Results DOW BETAMATE 1022DUS Material Code No Backing Plates Shear Strength Cohesive Failure Shear Strength Backing Plates Cohesive Failure MPa σ % σ MPa σ % σ 590Y-C 25 0.4 96 2 33 1.0 99 1 590Y-96 31 1.0 73 14 590R-12 34 1.2 99 0 590T-897 34 1.0 96 2 270E-35 13 0.4 0 0 29 1.0 0 0 270D-06 24 0.6 77 23 0% CF 50% CF 99% CF

Material Code Results DOW BETAMATE 73305GB No Backing Plates Shear Strength Cohesive Failure Shear Strength Backing Plates Cohesive Failure MPa σ % σ MPa σ % σ 590Y-C 23.4 0.8 58 19 36.4 0.8 96 4 590Y-96 30.2 1.2 5 0 590R-12 35.8 0.8 95 4 590T-897 34.7 35 10 2 270E-35 10.9 0.5 0 0 24.6 2.4 0 0 270D-06 21.2 0.8 2 3 0% CF 10% CF 99% CF

Results Three Adhesives

Results Three Adhesives

Results Three Adhesives BETAMATE 1488, with the lowest E-modulus, was the only adhesive to exhibit excellent cohesive bonding performance for all test materials except the thin gauge IF EDDS material. Lap shear performance using adhesives with a higher modulus was fair or poor, despite good adhesion at the steel/coating interface, suggesting that other coating and adhesive characteristics influenced the mode of failure. All test materials fell within acceptable variation of GA coated product and the low modulus adhesive appeared to compensate for subtle variations in the GA coated product.

Conclusions All 590 materials exhibited excellent adhesive bond strengths with all adhesives even when the mode of failure was less than optimal. The amount of cohesive failure decreased as the E-modulus of the adhesive increased. A low modulus, crash resistant adhesive has potential to be used with GA coated AHSS structures to reduce weight while maintaining or improving crash performance. The recommendation would remain to avoid joining GA IF EDDS steels with adhesives in crash sensitive applications.