Screening with accurate mass instruments coupled with LC



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News from EURL AO Ralf Lippold, Fabian Bäuerle, Heike Müller Svetlana Juschenko, Sabine Walter, Tanja Radykewicz, Benjamin Dambacher, Björn Hardebusch Stuttgart, 30 September 2015 1 / News from EURL AO

News from EURL AO Content of the Presentation Cleanup (LC-analysis) Screening with accurate mass instruments coupled with LC Method for less polar pesticides 2 / News from EURL AO

Cleanup (LC Pesticides) Since early summer 2015 Agilent offers a cleanup test kit for fatty matrices (EMR Kit) Agilent chemicals replace the typical QuEChERS-ingredients EMR dspe (composition?) instead of buffer and salts (4 g MgSO 4 ; 1 g NaCl; 0,5 g Na 2 Hcitrate x 6 H 2 O; 1 g Na 3 citrate x 2 H 2 O) EMR polish (mixture of MgSO 4 and 1 g NaCl) for drying the solvent Comparision: Cleanup according QuEChERS AO Cleanup according QuEChERS with Agilent EMR kit 3 / News from EURL AO

Cleanup: Proof applying thin layer chromatography Stationary phase: silica gel, 60 µm Mobile phase: petroleum ether / diethyl ether/ acetic acid (85/15/1.5; v/v/v) Spraying reagent: 10% phosphomolybdic acid in ethanol Heating: 2 min @ 150 C Shown by Fanny Hildmann at EPRW 2014 in Dublin German Official Method according 64 LFGB; No. L 13.00-27/2 Appendix A 4 / News from EURL AO

Thin-layer chromatography Solution front line cholesterol esters triglycerides free fatty acids free cholesterol Start line phospholipids Q kidney Agi kidney Q liver Agi liver Q: QuEChERS Agi: QuEChERS with Agilent sorbens 5 / News from EURL AO

Cleanup: what about the Pesticides Cleanup according QuEChERS AO Cleanup according QuEChERS with Agilent EMR kit Cleanup according SweEt (slightly modified by EURL AO) Spiking @ 0.010 mg/kg with 142 pesticides (calibration standard mix for qqq-analysis) Results (Screening with LC-q-ToF): QuEChERS AO: 136 pesticides detected (95.8 %) QuEChERS EMR kit: 136 pesticides detected (95.8 %) SweEt mod. EURL AO: 135 pesticides detected (95.1 %) 6 / News from EURL AO

Training of NRLs for Pesticides in Food of Animal Origin and Commodities with High Fat Content 28-29 September 2015, Freiburg, Germany Ralf Lippold Björn Hardebusch Tanja Radykewicz Benjamin Dambacher Karin Malisch Rainer Malisch Fabian Bäuerl Carolin Hauler Maria Schmitt Katrin Thoma

Cleanup Sample amount Extraction Clean-up Preparation before analysis QuEChERS for Food of Animal Origin 5 g matrix of interest (liquid whole egg, cow s milk, cheese, meat, honey ) 50 ml centrifuge tube Addition of internal standard: add 100 µl ISTD to both and spike one tube with 200 µl spiking solution, wait 10 min Addition of 10 ml water, shake or vortex (10 min) Addition of 10 ml ACN, shake or vortex (10 min) 4.0 ± 0.2 g MgSO 4 + 1.0 ± 0.05 g NaCl + 1.5 g Citrate salts (0,5 g Na 2 H-citrate x 6 H 2 O, 1.0 g Na 3 -citrate x 2 H 2 O) Shake vigorously for 10 min Centrifuge for 5 min at 2500 g (4000 rpm) 15 ml centrifuge tube filled with : 900 mg MgSO 4 + 150 mg PSA Add 6 ml supernatant Shake for 10 min Centrifuge for 5 min at 2500 g (4000 rpm) Transfer 2 times 1 ml into LC-vials Analysis LC-MS/MS + LC-MS-TOF 8 / News from EURL AO

Cleanup Sample amount Extraction Clean-up Preparation before analysis QuEChERS for Food of Animal Origin (Agilent chemicals) 5 g matrix of interest (liquid whole egg, cow s milk, cheese, meat, honey ) 50 ml centrifuge tube Addition of internal standard: add 100 µl ISTD to both and spike one tube with 200 µl spiking solution, wait 10 min Addition of 10 ml water, shake or vortex (10 min) Addition of 10 ml ACN, shake or vortex (10 min) Transfer 8 ml of ACN supernatant into the 15 ml dspe EMR-lipid centrifuge tube Shake vigorously for 10 min Centrifuge for 5 min at 2500 g (4000 rpm) Transfer supernatant into 15 ml centrifuge tube filled with: Final polish EMR-lipid (Magnesium sulfate, sodium chloride) Shake for 10 min Centrifuge for 5 min at 2500 g (4000 rpm) Transfer 2 times 1 ml into LC-vials Analysis LC-MS/MS + LC-MS-TOF 10 / News from EURL AO

Cleanup SweEt for Food of Animal Origin Sample amount Extraction 5 g matrix of interest (liquid whole egg, cow s milk, cheese, meat, honey ) 50 ml centrifuge tube Addition of internal standard: add 100 µl ISTD to both and spike one tube with 200 µl spiking solution, wait 10 min Addition of 10 ml water, shake or vortex (10 min) - (not for milk) Addition of 10 ml ethyl acetate Shake vigorously for 10 min 5.0 ± 0.2 g Na 2 SO 4 + 0.2 g C 18 + 0.2 g PSA Shake vigorously for 10 min Centrifuge for 5 min at 2500 g (4000 rpm) Preparation before analysis Transfer 2 times 1 ml into LC-vials Analysis LC-MS/MS + LC-MS-TOF 11 / News from EURL AO

Cleanup Challenges in life training ToF-results not availabe at the time beeing Strike of the Agilent LC-MS-q-ToF On Sunday, Jan Elias Hardebusch arrived in Freiburg 12 / News from EURL AO

Cleanup: Results achieved during the training 28./29. September 2015 13 / News from EURL AO

Screening Content of the Presentation Cleanup (LC-analysis) Screening with accurate mass instruments coupled with LC Method for less polar pesticides 14 / News from EURL AO

Screening Typical Instruments on the market ToF or q-tof coupled to LC or GC Orbitrap or q-orbitrap coupled to LC or GC 15 / News from EURL AO

Screening Application of accurate mass MS in Pesticide Residue Analysis 1. Qualitative Screening by using cut of limits (e.g. the Screening Detection Limit SDL or the Detection Capability (CCß) - 2002/657/EC) 2. Complementary technique to classical detectors Increase of available information for detected pesticides 3. Search for analytes of special interest (e.g. find by formular ) 4. Search for real unknown by the using databases 5. Evaluation of the sample background 16 / News from EURL AO 16

Screening Application of accurate mass MS in Pesticide Residue Analysis 1. Qualitative Screening @ SDL 2. Complementary technique to classical detectors 3. Search for analytes of special interest 4. Search for real unknown by the using databases Reporting possible in case of applying validated methods (requirement of ISO 17025!) Results of applications 3 and 4 are typical for internal use, only 17 / News from EURL AO 17

News from EURL AO 5. Evaluation of the sample background, e.g. by MFE Crayfish 3893 Matrix compounds Total Area 3E+7 Goat Cheese 3498 Matrix compounds Total Area 2.6E+7 Honey 3206 Matrix compounds Total Area 4575 Matrix compounds Total Area Sheep liver 3E+7 3.2E+7 18 / News from EURL AO 18

Screening 5. Evaluation of the sample background Principle Component Analysis (PCA) Information about similar background LC-QQQ: Pool of matrices for calibration possible? Co-Project together with EURL FV (Almeria, Spain) Goat Cheese Honey Crayfish Pepper Orange Thanks to Amadeo R Fernandez Alba and Ana Lozano Sheep liver 19 / News from EURL AO 19

Screening in Pesticides Residue Analysis Decision Qualitative Screening <-> Confirmatory Method Qualitative Screening Pesticides never found or few findings in Europe Detection @ 0.01 mg/kg (ß <= 5 %) Detection below MRL-level (not for MACCP) Confirmatory Method Pesticides frequently or sometimes found Pesticides with unsatisfying SDL 20 / News from EURL AO 20

Screening: LC-MS-Q-TOF Conditions HPLC Methode1290 Series Simple method for all analyts Injection volume 2-5 µl Column Zorbax Eclipse Plus C-18 HD, 150 x 2.1mm, 1.8 µm Gradient: solvent A = 5 mm NH 4 Formiate; solvent B = ACN Time (min) % B Flow (ml) 0 5 0.3 1 5 0.3 30 95 0.3 32.5 95 0.3 33 5 0.3 Q-TOF Method MSScan (sensitive scan) in 4 GHz-Modus Targeted MSMS (identification) Data base research (optimized for pesticides with RT) 21 / News from EURL AO

Workflow Screening EXAMPLE: EXPERIMENTAL DESIGN OF A VALIDATION STUDY (Eggs) Sample Treatment 241 analytes were spiked at 4 different levels 20 Blank matrices 10 different samples of hen s eggs 5 spiking levels 0 mg/kg / 0.005 mg/kg / 0.010 mg/kg / 0.020 mg/kg / 0.040 mg/kg Number of analyses In total 100 analyses (2 replicates of each sample analysed at 5 concentration levels) QuEChERS clean up LC-MS-ToF (ESI pos, only) Evaluation against own database 22 / News from EURL AO

Workflow Screening 23 / News from EURL AO

Workflow Screening 24 /News from EURL AO

Results of the Screening Validation Study (Egg) Results with LC-q-ToF (ß-error 5%) Results with LC-q-Orbitrap (ß-error 5%, analysis performed by Thermo) Details will be presented for egg and honey at RAFA (Prague) 25 / News from EURL AO

Screening Evaluation of retention times Retention time (egg study) Total number of RTs: 15718 Reproducebility conditions Repeatabiltiy conditions # +/- 0.1 min 14869 94,6% > 99 % # +/- 0.2 min 809 5,1% # outlier 40 0,3% << 0.1 % Retention time (honey study) Total number of RTs: 26832 Reproducebility conditions Repeatabiltiy conditions # +/- 0.1 min 25434 94,8% > 99 % # +/- 0.2 min 775 2,9% # outlier 623 2,3% << 0.1 % 26 / News from EURL AO

Less Polar Pesticides Content of the Presentation Cleanup (LC-analysis) Screening with accurate mass instruments coupled with LC Method for less polar pesticides 27 / News from EURL AO

Extraction for less polar pesticides at CVUA Freiburg Sample preparation example Mix 5 g (10% fat) of sample with sodium sulfate (~50 g) Soxtherm extraction with light petroleum Filtrate, evaporate to dryness Re-dissolve in ethylacetate/cyclohexane Take an aliquot of 5 ml for clean-up (containing ~0.5 g fat) clean-up 28 / News from EURL AO

Clean-up for GC-Analysis Clean up Addition of internal Standards 2,4,5-TCB Mirex, Triphenylphoshat, PCB 209 GPC (Bio Beads S-X3) small silica gel column (1.5 % water) Fraction 2 Toluene Fraction 3 Toluene / Acetone 95 + 5 Final volume 0.5 ml Ready for GC-analysis all according EN 1528 29 / News from EURL AO

GC-Analysis after Clean up according EN 1528 More often problems analysing liver Liver extract; HP 5 MS/MS 30 / News from EURL AO

Advantages- and Disadvantages of Method (EN 1528) Method established with high experiences Final extracts suitable for Gas-Chromatography combined with all GC-detection systems For MS-Measurement only few maintenance effort necessary (1-2 times a year), few liner changes 6-7 different solvents are used during the analysis procedure High solvent volume (~500 ml per analysis), recycling at CVUA Time consuming steps (2-3 working days per batch), esp. extraction step High costs for glassware and man power How to increase the efficiency (saving time and money)? How to increase the cleanup (liver!) 31 / News from EURL AO

Possible alternatives? QuEChERS - SweEt Co-extracted fat may lead to problems in GC analysis (especially SweEt) Low recovery rates for non-polar analytes (QuEChERS) 32 / News from EURL AO

Reproducibility: GC-MSMS of QuEChERS extracts Matrix: cream (frozen extract) 10 Injections Injection Deltamethrin Fenvalerate I Fenvalerate II 1 595 14625 9101 2 534 14129 7450 3 208 7461 3736 4 250 7432 4113 5 191 5426 3479 6 192 5564 2858 7 156 4994 3588 8 127 5500 2107 9 138 4596 1566 10 132 4283 1382 Mean 252 7401 3938 standarddeviation 169 3826 2496 cv [%] 67.2% 51.7% 63.4% 16000 14000 12000 10000 8000 6000 4000 2000 0 1 2 3 4 5 6 7 8 9 10 Deltamethrin Fenvalerate I Fenvalerate II {CAS # 51630-58-1} Loss of sensitivity no reproducibility with dirty extracts. Data obtained from test measurements on Agilent GC-MSMS 33 / News from EURL AO

Modification of existing method for pesticide residues Extraction procedure, modified Mixture of ethylacetate and cyclohexane used for extraction Combination with existing EN 1528 clean-up approach The extract should be ready to use for GPC clean-up No additional dilution or evaporation steps after extraction 34 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin 5 g sample + Internal Standards wait 10 min + 5 ml water + citrate buffer salts Shake 10 sec + 10 ml ethylacetate/ cyclohexane (1+1/v+v) Shake 10 min 35 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin + 10 g Na 2 SO 4 + 0.2 g PSA Shake 10 min Centrifuge (2500 g) Take 5 ml extract GPC-cleanup 36 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin Evaporate solvent Re-dissolve in isooctane silica gel column Evaporate Final volume 0.5 ml GC-MS/MS-Analysis 37 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin Extraction procedure, modified Mixture of ethylacetate and cyclohexane used for extraction Combination with existing EN 1528 clean-up approach The extract is ready to use for GPC clean-up No additional dilution - evaporation step after extraction Extraction efficient regarding extraction and time (Time reduced to 1.5-2 working days per batch) Cleanup like in original method -> no improvement 38 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin Z-sep+ was used during the extraction procedure resulting in cleaner extracts (visual control) For later tests the z-sep+ was layered over the silica gel after the GPC (it worked!) Extracts of liver Finally, z-sep+ is used after the GPC 39 / News from EURL AO

Less Polar Pesticides in Food of Animal Origin During routine analysis cases with dirty liver extracts occurred Working sequential for checking reasons can be very time consuming Designed experiment for checking effects 40 / News from EURL AO

Method for analysing less polar pesticide in food of animal origin - final modifications Effects During Clean Up (Optimizing 2) -80-60 -40-20 0 Umlösen und Reinigen zsep+ 20 40 60 80 TPP Aldrin Chlorbenzilat Dieldrin Endrin HCB Heptachlor gamma-hch (Lindan) Methoxychlor (p,p'-) Nitrofen S-421 alpha-hch beta-hch delta-hch Oxychlordan Endosulfansulfat DDE-o,p' DDE-p,p' DDT-o,p' DDT-p,p' DDD-o,p' DDD-p,p' alpha-endosulfan beta-endosulfan alpha-chlordane (cis) gamma-chlordane (trans) cis-heptachlorepoxid transheptachlorepoxid Endrin-Keton Bromocyclen trans-nonachlor Fenpropathrin Jodfenphos Chlorpyrifos Coumaphos Diazinon Fenthion Parathion Parathion-methyl Pirimiphos-ethyl Pirimiphos-methyl Pyrazophos Triazophos Chlorpyrifos-methyl Propetamphos Profenofos Fenthion-sulfon Azinphos-ethyl Quintozen Tecnazen Pendimethalin lambda-cyhalothrin cis-permethrin trans-permethrin Deltamethrin PCB 118 PCB 28 PCB 52 PCB 101 PCB 180 PCB 138 PCB 153 Triclosan-methyl Moschus-Xylol Moschus-Keton Cypermethrin (gesamt) Cyphenothrin (gesamt) Fenvalerate (gesamt) Cyfluthrin (gesamt) 41 / News from EURL AO

Method for analysing less polar pesticide in food of animal origin - final modifications Effects During Clean Up (Optimizing 2) -50-40 -30-20 -10 0 Elution 10 20 30 40 50 TPP Aldrin Chlorbenzilat Dieldrin Endrin HCB Heptachlor gamma-hch (Lindan) Methoxychlor (p,p'-) Nitrofen S-421 alpha-hch beta-hch delta-hch Oxychlordan Endosulfansulfat DDE-o,p' DDE-p,p' DDT-o,p' DDT-p,p' DDD-o,p' DDD-p,p' alpha-endosulfan beta-endosulfan alpha-chlordane (cis) gamma-chlordane (trans) cis-heptachlorepoxid transheptachlorepoxid Endrin-Keton Bromocyclen trans-nonachlor Fenpropathrin Jodfenphos Chlorpyrifos Coumaphos Diazinon Fenthion Parathion Parathion-methyl Pirimiphos-ethyl Pirimiphos-methyl Pyrazophos Triazophos Chlorpyrifos-methyl Propetamphos Profenofos Fenthion-sulfon Azinphos-ethyl Quintozen Tecnazen Pendimethalin lambda-cyhalothrin cis-permethrin trans-permethrin Deltamethrin PCB 118 PCB 28 PCB 52 PCB 101 PCB 180 PCB 138 PCB 153 Triclosan-methyl Moschus-Xylol Moschus-Keton Cypermethrin (gesamt) Cyphenothrin (gesamt) Fenvalerate (gesamt) Cyfluthrin (gesamt) 42 / News from EURL AO

Method for analysing less polar pesticide in food of animal origin 5 g sample + Internal Standards wait 10 min Centrifuge (2500 g) Cleanup Step Re-dissolve in isooctane silica gel column + 5 ml water + citrate buffer salts + 10 ml ethylacetate/ cyclohexane (1+1/v+v) + 10 g Na 2 SO 4 + 0,2 g PSA Shake 10 sec Shake 10 min Use 5 ml extract for GPC-cleanup Concentrate solvent Z-sep+ clean up Evaporate solvent Shake 1 min, filtrate Re-dissolve in cyclohexane Final volume 0.5 ml GC-MS/MS-Analysis Elute with toluene+aceton (95+5) 43 / News from EURL AO

Thin-layer chromatography of extracts (egg) for the GC measurement Solution front line cholesterol esters triglycerides free fatty acids free cholesterol phospholipids Start line S19 El 2(*) S19 El 3 (*) AO El 2 AO El 3 AO + ZrO2 - SG QuEChERS SweEt AO: El: SG: new EURL AO Methode Eluate Silica Gel ZrO 2 : Zirconium(IV)-oxid (*) Factor 4 less concentrated than the other extracts 44 / News from EURL AO

Analysis of samples Use of matrix matched calibration (using extracted liver expected to be free of pesticide residues) Improvement by using procedural calaibration (using blank matrix spiked before the first extraction step) Analysis performed using the Agilent 7890A with 7000B QQQ ( Pesticide Analyzer ) Backflush, installed 45 / News from EURL AO

TIC (MRM; extracts of liver after modifications) TIC demonstrates the enhanced cleanup of the modified AO method 46 / News from EURL AO

ECD: extracts of egg ECD demonstrates the enhanced cleanup of the modified AO method 47 / News from EURL AO

Method Validation (liver and egg) 1. About 60 less polar pesticides and contaminants Hexachlorbenzol HCB HCH, alpha- HCH, beta- Lindan gamma-hch HCH, deltatrans-nonachlor DDE, op- DDE, pp- DDT, op- DDT, pp- DDD, op- DDD, pp- PCB 28 PCB 52 PCB 101 PCB 153 PCB 138 PCB 180 PCB 118 Aldrin Dieldrin Heptachlor Heptachlorepoxid, cis- Heptachlorepoxid, trans- Endosulfan, alpha- Endosulfan, beta- Endosulfan-sulfat Chlordan, alpha(cis)- Chlordan, gamma(trans)- Oxychlordan Bromocyclen; Bromodan S 421 Moschus-Xylol Moschus-Keton Endrin Delta-Ketoendrin Iodofenphos Methoxychlor Nitrofen Triclosan-methyl Pendimethalin Tecnazen Quintozen Fenpropathrin Lambda-Cyhalothrin, Cyphenothrin cis-permethrin trans-permethrin Cyfluthrin, Cypermethrin, Fenvalerat und Esfenvalerat, Deltamethrin Chlorpyrifos-methyl Parathion-methyl Pirimiphos-methyl Chlorpyriphos(-ethyl) Parathion(-ethyl) Pirimiphos-ethyl Fenthion 48 / Pesticides in Liver <-> GC-MS/MS

Method Validation 1. About 60 less polar pesticides and contaminants 2. 4 levels of spiking (plus blank liver) 3. 2 different staff for the cleanup procedures 4. Each staff with 3 replicates at 4 concentrations 3 3 6 replicates per level 49 / News from EURL AO

Results Liver (0.1 8 µg/kg as LOD) Lambda-Cyhalothrin Matrix matched calibration Pirimiphos-methyl Pirimiphos-ethyl 7 % 7 % 93 % 3 % 83 % Fenthion Recovery rates of the analytes: 70-120 % 100 ± 10 % < 70 % 70-90 % 110-120 % 50 / News from EURL AO

Results Egg (0.1 10 µg/kg as LOD) *Includes Tralomethrin Procedural Calibration LOD [µg/kg] Pesticides 0.1 DDE, op-, DDT, op-, DDT, pp-, Heptachlorepoxid, trans-, Quintozen 0.2 Aldrin, Bromocyclen; Bromodan, Chlordan, alpha(cis)-, Chlordan, gamma(trans)-, op-ddd, pp-ddd, delta-ketoendrin, Dieldrin, alpha-endosulfan, beta-endosulfan, Endosulfan sulfat, alpha-hch, beta-hch, delta-hch, cis-heptachlorepoxid, Hexachlorbenzol, Lindan, Moschus-Xylol, Oxychlordan, PCB 101, PCB 118, PCB 138, PCB 180, PCB 28, PCB 52, Prallethrin, trans-nonachlor 0.3 0.4 Heptachlor, Iodofenphos, pp-dde, Endrin, Nitrofen, PCB 153, Pendimethalin, Triclosanmethyl, Fenthion-Sulfon 0.5-1.0 Azinphos-ethyl, Chlorpyrifos-methyl, Chlorpyriphos(-ethyl), Diazinon, Methidathion, Parathion(-ethyl), Parathion-methyl, Pirimiphos-ethyl, Pirimiphos-methyl, Profenofos, Propetamphos, Pyrazophos, Triazophos, S 421, Fenthion, Piperonylbutoxid, Bifenthrin, Methoxychlor, Moschus-Keton, Fenpropathrin, Fenvalerat Esfenvalerat (sum), Flucythrinat (2 isomeres) > 1.0 5.0 Methothrin, Chlorbenzilat, Cyfluthrin (total), Cypermethrin (total), Tetramethrin, Cyhalothrin (total), Coumaphos, Allethrin, cis-permethrin, trans-permethrin, Cyphenothrin > 5.0 10 Empenthrin, Resmethrin (total), tau-fluvalinat (2 Isomeres), Pyrethrum Pyrethrine (sum), Deltamethrin*, Phenothrin No final validation: Fenthion-ethyl, Kadethrin, Paraoxon-methyl, Tefluthrin, 51 / News from EURL AO

Method for analysing less polar pesticide in food of animal origin: LIVER 5 g sample + Internal Standards wait 10 min Centrifuge (2500 g) Cleanup Step Re-dissolve in isooctane silica gel column + 5 ml water + citrate buffer salts + 10 ml ethylacetate/ cyclohexane (1+1/v+v) + 10 g Na 2 SO 4 + 0,2 g PSA Shake 10 sec Shake 10 min Use 5 ml extract for GPC-cleanup Concentrate solvent Z-sep+ clean up Evaporate solvent Shake 1 min, filtrate Re-dissolve in cyclohexane Final volume 0.5 ml GC-MS/MS-Analysis 52 / News from EURL AO

Method for analysing less polar pesticide in food of animal origin: Egg, Milk - Babyfood, Muscle 5 g sample + Internal Standards wait 10 min Centrifuge (2500 g) X Cleanup Step Re-dissolve in isooctane silica gel column + 5 ml water + citrate buffer salts + 10 ml ethylacetate/ cyclohexane (1+1/v+v) + 10 g Na 2 SO 4 + 0,2 g PSA 53 / News from EURL AO Shake 10 sec Shake 10 min Use 5 ml extract for GPC-cleanup Concentrate solvent Z-sep+ clean up Evaporate solvent Shake 1 min, filtrate Re-dissolve in cyclohexane Final volume 0.5 ml GC-MS/MS-Analysis

Method for analysing less polar pesticide in food of animal origin: HONEY 5 g sample + Internal Standards wait 10 min Centrifuge (2500 g) X Cleanup Step Re-dissolve in isooctane silica gel column + 5 ml water + citrate buffer salts + 10 ml ethylacetate/ cyclohexane (1+1/v+v) + 10 g Na 2 SO 4 + 0,2 g PSA 54 / News from EURL AO Shake 10 sec Shake 10 min Use 5 ml extract for GPC-cleanup?X? X Concentrate solvent X Z-sep+ clean up Evaporate solvent Shake 1 min, filtrate Re-dissolve in cyclohexane Final volume 0.5 ml GC-MS/MS-Analysis

Final Thank you for your attention! GC-Liner after tests and the liver validation study 55 / News from EURL AO