Environmental radioactivity during 50 years

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Downloaded from orbit.dtu.dk on: Jan 27, 2017 Environmental radioactivity during 50 years Nielsen, Sven Poul Publication date: 2013 Link to publication Citation (APA): Nielsen, S. P. (2013). Environmental radioactivity during 50 years [Sound/Visual production (digital)]. NKS Workshop on Radioanalytical Chemistry, Roskilde, Denmark, 02/09/2013, http://www.nks.org/en/seminars/presentations/nks-b_radioanalysis_workshop_2-6_september_2013.htm General rights Copyright and moral rights for the publications made accessible in the public portal are retained by the authors and/or other copyright owners and it is a condition of accessing publications that users recognise and abide by the legal requirements associated with these rights. Users may download and print one copy of any publication from the public portal for the purpose of private study or research. You may not further distribute the material or use it for any profit-making activity or commercial gain You may freely distribute the URL identifying the publication in the public portal? If you believe that this document breaches copyright please contact us providing details, and we will remove access to the work immediately and investigate your claim.

Environmental radioactivity during 50 years Sven P. Nielsen

Investigations of man-made radioactivity in the Danish environment from 1957 2 DTU Nutech, Technical University of Denmark

Atmospheric nuclear weapons tests Atmosfæriske atomprøvesprængninger 180 Global pollution from atmospheric nuclear weapons tests: fission products, activation products, fissile material and tritium Mt/år 160 140 120 100 80 60 40 Fusion Fission 20 0 1945 1948 1951 1954 1957 1960 1963 1966 År 1969 1972 1975 1978 DTU Nutech, Technical University of Denmark

Radioecological sensitivity Studies covering Air, water, soil Grain, bread Grass Vegetables and fruit Sea plants Milk, meat, fish Total diet Human body, bone Radioecological sensitivity is the time integral of quantities of the sample type from a quantity of the radionuclide deposited Example for Cs-137 in Danish cow s milk 2.0 Bq/L d per Bq/m 2 4 DTU Nutech, Technical University of Denmark

Strontium-90 and caesium-137 Fission products of particular importance due to long half lives and significant uptake in food chains 5 DTU Nutech, Technical University of Denmark 2012-10-31

Aerosols Monitoring of radioactivity in air is based on aerosol collectors located in Haderslev, Allinge and Risø. Air is sampled at flow rates of 500-2000 m 3 /h through organic filters retaining particles Filters are changed weekly and analysed for short-lived radionuclides first and later for longer lived radionuclides, particularly 7 Be, 210 Pb, 90 Sr, 137 Cs. Risø DTU Nutech, Technical University of Denmark

Radioactivity in Air at Risø 1.E+04 1.E+03 Atmospheric nuclear weapons tests 1945-1980 Chernobyl, 1986 Fukushima, 2011 CONCENTRATION (µbq/m 3 ) 1.E+02 1.E+01 1.E+00 Sr 90 Cs 137 1.E 01 1.E 02 1955 1965 1975 1985 1995 2005 2015 YEAR 7 DTU Nutech, Technical University of Denmark

Precipitation Precipitation is collected at Risø and 10 other locations in Denmark and analysed for content of Sr-90 and Cs-137 8 DTU Nutech, Technical University of Denmark

Milk, potatoes, vegetables and total diet 9 DTU Nutech, Technical University of Denmark

Cereals: rye, oats, wheat, barley 10 DTU Nutech, Technical University of Denmark

Stream, lake and ground water 11 DTU Nutech, Technical University of Denmark

Sea water and plants 10 E 11 E 12 E 13 E Kattegat-413 Kattegat SW Hesselø Kullen Øresund, N, B 56 N Øresund, N, A Asnæs rev Halskov rev Øresund, S Møen 55 N Langeland bælt Femern bælt Gedser odde DTU Nutech, Technical University of Denmark

Caesium-137 in fish/cod 100 Koncentration (Bq/kg frisk vægt) 10 1 0.1 Færøerne Grønland Nordsøen Kattegat Østersøen 0.01 1960 1970 1980 1990 2000 2010 År DTU Nutech, Technical University of Denmark

Humans Employees at Risø monitored for radiocaesium and tritium Human bone samples received from hospitals (with difficulty) 14 DTU Nutech, Technical University of Denmark

External exposure 15 DTU Nutech, Technical University of Denmark

Radioactive contamination in Denmark Poster in building 204 shows concentrations of strontium-90 and caesium-137 in air, precipitation, milk and grass at Risø and in Denmark since the 1950 s Including input from the Fukushima accident in Japan in 2011 16 DTU Nutech, Technical University of Denmark

Why monitor environmental radioactivity? EURATOM Treaty: Health and safety matters - Obligation of EC Member States to monitor levels of radioactivity in air, soil and water and to ensure compliance with basic standards Helsinki Convention: Contracting Parties undertake to prevent and eliminate pollution of the marine environment of the Baltic Sea Area caused by harmful substances from all sources Study man-made and naturally occurring radionuclides in the environment to document baseline levels and increase knowledge on behaviour and processes Expertise available for emergency purposes in case of accidents/incidents involving release of radioactivity to environment Improve radiological assessment models in decision support systems used by authorities in case of accidents Useful platform for research and development of existing and new analytical methods and application of these in other areas 17 DTU Nutech, Technical University of Denmark