The Future of the Nuclear Fuel Cycle



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The Future of the Nuclear Fuel Cycle An Interdisciplinary MIT Study Ernest J. Moniz Cecil and Ida Green Professor of Physics and Engineering Systems Director, MIT Energy Initiative

Study Participants Co-chairs: Executive Director: Mujid Kazimi and Ernest J. Moniz Charles W. Forsberg Steve Ansolabehere John M. Deutch Michael J. Driscoll Michael W. Golay Andrew C. Kadak John E. Parsons Monica Regalbuto George Apostolakis Pavel Hejzlar Eugene Shwageraus Blandine Antoine Guillaume De Roo Bo Feng Laurent Guerin Isaac Alexander Matthews Lara Pierpoint Behnam Taebi Keith Yost

Advisory Committee Phil Sharp, Chairman, Resources for the Future James K. Asselstine, Barclays Capital Jacques Bouchard, Commissariat a l energie atomique, France Marvin Fertel, Nuclear Energy Institute Kurt Gottfried, Union of Concerned Scientists John Grossenbacher, Idaho National Laboratory Jonathon Lash, World Resources Institute Richard A. Meserve, Carnegie Institution for Science Cherry Murray, Harvard University John W. Rowe, Exelon Corporation Maxine L. Savitz, U.S. National Academy of Engineering Steven R. Specker, Electric Power Research Institute John H. Sununu, JHS Associates

Electric Power Research Institute Idaho National Laboratory Nuclear Energy Institute Areva GE-Hitachi Westinghouse Energy Solutions Nuclear Assurance Corporation Sponsors

For the next several decades, once through fuel cycle using light water reactors is the preferred economic option for the U.S. Accelerate implementation of first mover incentive program No shortage of uranium resources Scientifically sound methods to manage spent nuclear fuel (SNF) Resource extension and waste management benefits of limited recycling (MOX) are minimal Fuel cycle transitions take a long time: many LWRs and little difference in total transuranic inventories or uranium needs in this century in standard closed fuel cycle scenario

Planning for long term managed storage of SNF for about a century should be integral for fuel cycle design Can and should preserve options for disposal, reprocessing, recycle Why? Major uncertainties for informed choices: Societal: NP growth? Nonproliferation norms?... Technical: fast or thermal reactors? Conversion ratio? Waste management benefits? SNF as resource or waste?... Start moving SNF from shut-down reactors Move to centralized managed storage: not for economics or safety

A key technical point: CR=1 sustainable and has advantages High CR constrains choices: Pu-initiated fast reactor Rooted in uranium resource expectations Important technology choices made available with CR=1 LEU startup of fast reactor? SNF as waste? Saves uranium and lowers enrichment needs! Thermal reactors for closed fuel cycle? Economics vs fast reactors?

Waste management: geological disposal needed for any choice Systematically develop geological disposal, with public process Integrate waste management with fuel cycle design: waste stream requirements as important as what s recycled to reactor Develop risk-informed waste management system: composition not source Establish quasi-government waste management organization with sufficient authorities not recognizable in US program to date Site selection in concert with governments/communities Management of funds Negotiate SNF/waste removal with owners Engage policy/regulatory bodies on fuel cycle choices and waste Continuity in management

Nonproliferation and the fuel cycle: principally institutional Actively pursue fuel leasing with financial incentives and fixed term renewable commitment Absence of waste management program constrains options Technology choices have some impact: e.g., U-fed fast reactor scenario reduces U enrichment needs in second half of century

Commercial nuclear technology introduction has a long time constant, calling for strong RD&D program now: about $1B/yr DOE 2010 roadmap a good start LWR R&D important/ e.g., innovation hub on advanced simulation About a third for research infrastructure Large scale demonstrations in time

MIT Future of the Nuclear Fuel Cycle Study Uranium Resources and SNF Storage Charles Forsberg Executive Director MIT Nuclear Fuel Cycle Study Massachusetts Institute of Technology 77 Massachusetts Ave; Bld. 42-207a; Cambridge, MA 02139 Tel: (617) 324-4010; Email: cforsber@mit.edu September 16, 2009 MIT Center for Advanced Nuclear Energy Systems

12 Finding: Uranium Resources There is no shortage of uranium that might constrain future commitments to build new nuclear plants for much of this century Recommendation An international program should be established to enhance understanding and provide higher confidence in estimates of uranium costs versus cumulative uranium production

Uranium needs Uranium Cost Assessment ~200 tons per year for a 1000-MW(e) nuclear reactor 2 to 4% of the cost of nuclear electricity Uranium prices have small impacts on electricity prices We evaluated the costs of uranium mining versus cumulative worldwide uranium production. Inputs: Uranium resource estimates versus ore grade Economics of scale Technological learning over time Best estimate of 50% increase in uranium cost if: Nuclear power grows by a factor of 10 worldwide Each reactor operates for a century 13

1998 Dollars per Metric Ton Prices of 25 Metals Over a Century Uranium is a Metal: Similar Cost Trends For Most Metals 14 Inflation Adjusted Year

15 Spent Nuclear Fuel Management Finding SNF storage reduces repository costs and performance uncertainties. Fuel cycle transitions require a half century or more. Storage provides time to decide whether LWR SNF is a waste or resource Recommendation Planning for long term interim storage of spent nuclear fuel on the scale of a century should be an integral part of nuclear fuel cycle design

THERMAL POWER (W/MTIHM) Repository Programs Store SNF to Reduce Repository Size, Cost, and Performance Uncertainties Decay heat decreases with time, planned storage times are 40 to 60 years Sweden and France built SNF storage facilities in the 1980s for this purpose Proposed U.S. YMR had implicit storage system Fill repository over 30 years Operate ventilation for 50 additional years long-term storage 2000 1000 100 1.21X Sr + Cs 1.31X SPENT FUEL LESS Sr AND Cs 1.42X ACTINIDES IN SPENT FUEL ACTINIDE-FREE HIGH-LEVEL WASTE BASIS: PWR FUEL 3.2 wt % 235U 33 GWd/MTIHM 1.0 MTIHM TOTAL SPENT FUEL 10 10 100 1000 3X 129X DECAY TIME AFTER DISCHARGE (years) 16

It Takes 50 to 100 Years for Fuel Cycle Transitions 17 Transition from Light-Water Reactor to Fast Reactor Closed Fuel Cycle (2.5% Growth Rate)

18 It Will Be Decades Before We Know If LWR SNF Is a Resource or Waste LWR SNF has a high energy content Equivalent to super Strategic Petroleum Reserve LWR SNF could be a waste Alternative strategies to start fast reactors with sustainable fuel cycles using low-enriched uranium Alternative strategies may have lower costs

SNF at Decommissioned Sites Finding: The burden of SNF storage is small at an operating site This is not true for decommissioned sites where there are no longer the normal reactor operations associated with SNF handling, storage, and security. SNF storage limits reuse of these sites Recommendation We recommend that the U.S. move toward centralized SNF storage sites starting initially with SNF from decommissioned sites and in support of a long-term SNF management strategy 19

20 SNF Storage Options Finding: Either distributed storage (at reactor), centralized long-term storage, or storage in a repository is technically sound Recommendation An RD&D program should be devoted to confirm and extend the safe storage and transportation period

Systems Analysis: Fuel Cycle Options and Outcomes Mujid S. Kazimi Professor of Nuclear and Mechanical Engineering Director of Center for Advanced Nuclear Power Systems September 16, 2010 Briefing on MIT Study on Future of the Nuclear Fuel Cycle Center for Strategic and International Studies

Objective: Dynamic Simulation of the Nuclear Energy System Examine implications of a reasonable range of nuclear energy growth rates in the US on various nuclear fuel cycle options over this century. Key Questions: How would various fuel cycle options impact demand for nuclear fuel, mined or recycled? What is the impact of introducing recycling on the amounts of stored spent fuel, TRU and wastes to be sent to repositories? What parameters have the largest impact on demand for U, fuel cycle industrial infrastructure and spent fuel storage needs?

Fuel Cycle Options Base cases in red italics Once Through: Build ALWR/ Current Burnup (50 MWD/kg) Limited Thermal Reactor Recycle: PUREX-based one time recycling of U-Pu as mixed oxides (MOX) to LWRs Fast Reactor Recycle of all transuranics, TRU(metallic fueled reactors studied by ANL and GE): TRU to self-sustaining FR (Conversion Ratio =1) TRU recycle in fast burner ABR (with low CR = 0.75) TRU recycle in fast breeder FBR ( with CR = 1.23) Other cycle options have been considered.

Fuel Cycle Key Assumptions Nuclear power will grow to 115 GWe by 220; after 2020 at rates between 1% and 4%. Maximum allowed installed capacity is 1000 MWe. Dates for introduction of and lifetime of various options: Recycling of LWR spent fuel (MOX) 2025, 2040 Fast reactors and their fuel recycling 2040, 2060 FR Recycling plants are built to match reactor build schedule Reactor life time is 60 years. Recycling plant lifetime is 40 years Infrastructure constraints applied to recycling technology: Minimum SNF cooling time of 5 yrs (10 years), 1yr of reprocessing, and 1 yr of fuel manufacturing. Minimum lifetime capacity factor of recycling plant is 80%. LWR fuel recycling plant size: 1000MT/yr, can be added every 4 years prior to 2050, 2 years after 2050. FR recycling plant size 200MT/yr for burners and 500MT/yr for breeders; can be added every 2 years prior to 2050, then every 1 year U is recycled for all options.

Installed Capacity in GWe LWRs will play a major role throughout this century Fast reactor conversion ratio beyond 1.0 may not be helpful Growth Rate Fuel Cycle By 2050 By 2100 OTC 166 269 1.0% MOX 41 32 2.5% 4.0% FR* 20;22; 20 234; 236; 234 OTC 250 859 MOX 41 91 FR* 20; 23; 21 259; 345; 391 OTC 376 1,001** MOX 41 117 FR* 20; 23; 21 400; 521; 540 * Results are for conversion ratios = 0.75; 1.0; 1.23 ** Cap Reached in 2088

Installed LWR Capacity for the 2.5% growth case LWR with once through fuel cycle will grow under all options

Cumulative Demand for Uranium (1M MT) MOX has little effect, and fast reactors take decades to cause a real difference Growth Rate Fuel Cycle By 2050 By 2100 OTC 1.03 2.93 1.0% MOX 0.88 2.34 FR 0.98; 0.97; 0.98 1.77; 1.75; 1.77 OTC 1.26 5.86 2.5% 4.0% MOX 1.11 4.86 FR 1,21; 1.21; 1.21 4.16; 3.78; 3.76 OTC 1.56 8.11 MOX 1.41 6.77 FR 1.51; 1.51; 1.51 5.80; 5.34; 5.34

Required LWR Spent Fuel Reprocessing Capacity for the 2.5% Growth Case More capacity needed for lower conversion ratio reactors

Total TRU in system for 2.5% case Recycling has a modest effect on total TRU in the system. Total TRU = TRU In Reactors + Cooling and Interim Storage + Repository

Total TRU in the System Most TRU is in cooling storage and in fast reactor cores

What if we start fast reactors with medium enrichment uranium rather than plutonium? Both EBR-II and Russian BN-60 were started with highly enriched uranium (about 60%). Cores were small and not optimized for U startup. Recent work at MIT (Prof. Driscoll and Dr. Shwageraus) indicate that medium enriched uranium (under 20%) startup of a self-sustaining reactor is possible when an effective reflector is used (like MgO).

Uranium Requirements for LWR and for FR Startup For the base case of 2.5% Allows more rapid fast reactor penetration. Avoids recycling of LWR spent fuel which has only low fissile content. Reduces overall SWU capacity needed. Implications of cost of FR, and disposition of LWR spent fuel remain as open questions.

Conclusions -1 The controlling factors in the transition to advanced reactors with recycling: Rate of demand growth Availability of transuranics (TRU) from discharged fuels A smaller role for industrial capacity for FR fuel recycle and manufacture LWRs will have a major role in nuclear energy in this century, even after introduction of advanced reactors. Recycling will have limited impact on natural uranium consumption in this century: MOX starting in 2025 will have little impact (less than 10% if only Pu or TRU are used, less than 20% if U is also recycled) Fast reactors starting in 2040 will lead to about 30% reduction.

Conclusions -2 Recycling does not lead to appreciable reduction of TRU in total energy system, but leads to significant reduction in the amount of TRU destined to the repository in the short term. A repository is still needed. Options to start fast reactors on Uranium exist, and may be advantageous to U consumption. Self-sustaining reactors, with conversion ratio of 1.0 offer advantages for transition to a closed system. Choice of sodium reactors to maximize conversion ratio may not offer the optimum path forward. Several options for fast spectrum reactors, e.g. water cooled hard spectrum reactors, may reduce the cost of a sustainable nuclear energy system.

35 Questions 35