Validation of AirGIS - a GIS-based Air Pollution and Human Exposure Modelling

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Validation of AirGIS - a GIS-based Air Pollution and Human Exposure Modelling Traffic Traffic characteristics System Emissions Diurnal variation in traffic (TRF) GIS Addresses ID Exposure window GIS Buildings Building height Construction year Urban Landscape Model.CPR_year ID Exposure window.str_year ID Street configuration Traffic data.dbf Statistics (min, max) Fuel properties Car fleet data Mileage data Win OSPM Output Per year Average time-series Optional vehicle composition (TCM) Access Output summariz e for ID for exposure window Matthias Ketzel, Ruwim Berkowicz, Martin Hvidberg, Steen Solvang Jensen National Environmental Research Institute, Aarhus University, Denmark, and Ole Raaschou-Nielsen GIS Roads ADT (/5 year interval) Travel speed Street type Construction year GIS Land Use data Land use per hectar Emissions NewGridxy SumKmGrid UrbEmi Institute of Cancer Epidemiology, Copenhagen, Denmark UBM Background data Meteorological Regional air pollution Land use Urban Air pollution Regional backg. Urban backg. Meteorolog y Wind Temp Radiation THOR model system DMU measurements

Outline Introduction Motivation Model description Validation sources of error results hourly variation daily averages monthly Conclusions Funding provided by project Airpolife (Air Pollution in a Life Time Health Perspective) Danish Centre of Excellence on Air Pollution and Health 2004-2008 http://www.airpolife.dk/

Motivation Model estimates are useful for e.g.: assessment of compliance with air quality standards, for validation and optimisation of emission reduction strategies, for estimation of the personal exposure of groups of individuals in air pollution epidemiological studies for air pollution forecast and information of the public. AirGIS system ambient air quality levels with: high temporal resolution hours high special resolution - address

Spatial variation described by AirGIS street increment (str) modelled by OSPM concentration Local increment (loc) Street level concentration ( mod ) exposure points urban increment (urb) modelled by UBM or SUB (or measurements) regional background concentration ( r ) measured at Lille Valby / Keldsnor or modelled by THOR system // DEHM-REGINA city distance Urban background concentration ( b ) http://www.dmu.dk/international/air/models/airgis

AirGIS Street Configuration Describing the local horizon To allow calculations for different meteorological conditions the building height is determined in 12 discrete intervals, equally distributed on either side of the street. Modified from Hertel, O. 2006 From: AirGIS

AirGIS Base data Traffic Each street holds information about the local traffic. ADT: Avg. Daily Traffic (cars/day) in 5-years intervals from 1960 till today. Road construction year Street type (A..F) Allowed speed Actual speed

AirGIS Base data Buildings Each building holds information about itself. Building height Building construction year

AirGIS Input data Exposure points Each exposure point (EP) holds information about itself. Time start / stop Receptor height Transport mode Person travle speed Working hours, e.g. 9am 5pm Weekend days, e.g. Sat. Sun.

AirGIS - temporal variation and pollutants temporal variation hourly (basic calculation unit) daily averages monthly averages exposure periods (split in max. 1 year parts) Pollutants NO x, NO 2, O 3, CO, benzene, PM 10 and PM 2.5 NOx and CO for historic emissions back to 1960

Validation results sources of errors permanent monitoring stations HCOE (bg), Jagtvej, H.C. Andersens B. annual / daily / hourly childhood cancer campaign 204 addresses in Greater Copenhagen area 6 x 4 weeks of NO 2 averages

Sources of errors Input data background concentrations meteorology street configuration (W, H, location of buildings) traffic data (traffic volume, composition) fleet composition (age, technology EURO 1 / 2 etc.) emission factors (g per km, depending on speed) Dispersion model Front door concentration correct measure for exposure? right pollutant? positive relation with health effect -> still might be right for wrong reason no correlation found -> still method might be OK, just an error in some data, or one of the many steps

Validation results annual means for NO 2 JGTV Jagtvej, Copenhagen, HCOE - urban background Reg - regional background Obs observations, mod - model results. 35 30 25 NO2 in ppb 20 15 10 5 40µg/m3, EU Limit Value (=21ppb) NO2_str_JGTV_obs NO2_b_HCOE_obs NO2_Reg_obs NO2_mod_vari.DirectNO2 NO2_mod_5%DirectNO2 NO2_b_mod (UBM) 0 1988 1990 1992 1994 1996 1998 2000 2002 2004

Share of direct NO 2 emissions is increasing observed Jagtvej Share (in %) of direct NO 2 emissions 30 25 20 15 10 observed HCAB JGTV New Tab 23.4%PasDie JGTV New Tab 40%PasDie JGTV New Tab 60%PasDie MZ MZ+SCR MZ+SCRall modelled observed 5 0 1995 2000 2005 2010 2015 2020

Share of direct NO2 emissions is increasing Direct NO 2 emissions (% of NO x ) from different vehicle classes, based on literature data earlier 3-15%, now up to 45% due to CRT particle filters red: COPERT Før EURO EURO I EURO II EURO III EURO IV EURO V EURO VI Benzin personbiler 3 5 5 5 5 5 5 Diesel personbiler Taxi Diesel varebiler 15 15 15 30 40 40 20 Diesel lastbiler Diesel busser 8 8 8 8 45 20 20 4 4 4 3 3 3 2 11 11 11 25 55 5-70 5-70 1 11 11 14 14 10 10 35(+CRT) Sources: COPERT 4 Handbook Aug. 2007, U. Lambrecht IFEU 2008

Validation results monthly means performance of the two background models Urban Background Model (UBM) simplified urban background procedure (SUB) modelled (open symbols) and observed (full) NOx concentration in ppb 30 25 20 15 10 NOx_b_HCOE_obs NOx_b_UBM_mod NOx_b_SUB_mod NOx_reg_KELD_obs 5 0 1998 1999 2000 2001 2002 2003 2004 2005 2006

Validation results - statistics monthly means (ppb) during 1998-2005 Av= average, CoV= coefficient of variation Corr (R ) = correlation coefficient R, model vs. observed Location Method NOx NO2 O3 CO Av CoV Corr(R) Av CoV Corr(R) Av CoV Corr(R) Av CoV Corr(R) Keldsnor r_obs 5.7 0.38 4.8 0.41 30.2 0.26 THOR r_mod 7.1 0.17 0.71 6.3 0.17 0.60 26.0 0.27 0.92 HCOE u_obs 15.1 0.26 11.8 0.20 25.1 0.27 0.28 0.24 HCOE u_ubm (r_obs) 16.1 0.27 0.84 11.9 0.19 0.80 23.9 0.34 0.93 0.19 0.20 0.80 HCOE u_sub (r_obs) 13.6 0.23 0.79 10.8 0.19 0.75 24.8 0.32 0.92 0.28 0.16 0.82

Validation results daily means daily street concentrations of NOx, 2003, mod vs. obs (modelled background) Time-series, mod and obs daily urban background NOx concentrations modelled NOx in ppb 200 150 100 50 0 NOX_str_mod(OSPM) NOX_b_mod(UBM) y = 0.8128x + 8.102 R 2 = 0.7615 0 50 100 150 200 observed NOx_str in ppb meas/mod in ppb 60 50 40 30 20 10 NOx_b_mod(UBM) NOx_b_obs NOx_r_mod (THOR) NOx_r_obs 0 28-12-1999 11-01-2000 25-01-2000 08-02-2000 22-02-2000 07-03-2000 21-03-2000 04-04-2000 18-04-20

Validation results hourly data scatter plot average diurnal variation NOx_street-background (µg/m 3 ) 500 450 y = 0.697x + 16.656 R 2 = 0.7419 400 NOX_str_obs NOX_str_mod NOX_b 350 300 140 120 Modelled 250 80 200 60 150 40 20 100 0 50 0-100 0 100 200 300 400 500 600 700 Observed NOx in µg/m3 100 1 3 5 7 9 11 13 15 17 19 21 23 Hour of day

Validation results 204 streets Childhood Cancer project (Raaschou-Nielsen et al. 2000) each street 6 x 4 weeks passive sampled NO 2 model results from 2000 based on input data from questionnaires new calculations using the automated routines in AirGIS to create the input data Greater Copenhagen 70 60 questionnaires data AirGIS vers2, 08/2006 y = 1.0928x + 3.8261 R 2 = 0.8167 50 y = 0.9396x + 4.851 R 2 = 0.7821 Copenhagen NO2 modelled in µg/m 3 40 30 20 10 0 0 10 20 30 40 50 60 National Environmental Research NO 2 measured Institute, in µg/muniversity 3 of Aarhus

Validation results 204 streets Childhood Cancer project (Raaschou-Nielsen et al. 2000) 70 y = 1.0928x + 3.8261 R 2 = 0.8167 60 50 y = 0.9396x + 4.851 R 2 = 0.7821 NO 2 modelled in µg/m 3 40 30 20 10 0 questionnaires data AirGIS vers2, 08/2006 Hitrate FAC2 0 10 20 30 40 50 60 Hitrate Fac2 question. 0.453 0.952 AirGIS 0.536 0.951 National Environmental Research NO 2 Institute, measured University in µg/mof 3 Aarhus

Other examples for AirGIS application Geograpgic distribution of exceedances of NO2 limit value exposure to air pollution during travelling

Geographic distribution of exceedances About 80 exceedances of NO 2 limit value out of 138 streets in 2010 NO2 rsmiddel i 2010 ( ᅤg/m3) 18-29 29-40 40-44 44-52 52-63 ᅤDT 25-3802 3803-10595 10596-17799 17800-28114 28115-54781 N

Calculation of Air pollution along a route in AirGIS system

Conclusions The air pollution and human exposure modelling system, AirGIS, has been validated against observations at permanent monitoring locations. The system shows a good performance for long-term averages (annual and monthly averages). AirGIS also performs well for short-term averages (hourly and daily). High correlation coefficient 0.84 and 0.79 for NOx, for UBM and SUB respectively. Also for other pollutants the background models show high correlations and reproduce both the averages and the variation in the data expressed as coefficient of variation (CoV= ratio of standard deviation and average). AirGIS is therefore well suited for air pollution and exposure assessment in epidemiological studies.