Epoxy Curing Agents and Modifiers



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Epoxy Curing Agents and Modifiers 2489 Curing Agent DESCRIPTION 2489 curing agent is a low-color cycloaliphatic amine adduct intended for use with liquid epoxy resins. It has a very low viscosity which imparts low mixed viscosity in epoxy systems and reduced need for diluents. 2489 curing agent gives very rapid development of physical properties at ambient and low temperatures for a fast return to service, while maintaining longer working life than conventional fast cure hardeners. It yields formulations with good waterspot resistance, resistance to amine blush and chemical resistance. 2489 curing agent utilizes state-of-the-art adduct technology to provide a favorable combination of properties for formulating a variety of civil engineering and coating materials. ADVANTAGES Very low viscosity and mixed viscosity in epoxy systems Rapid cure and property development at ambient and low temperatures Good working life/cure speed balance Good resistance to blush and waterspotting Good chemical resistance APPLICATIONS Decorative and industrial flooring Chemically resistant high-solids coatings Mortars and grouts Sealers and primers STORAGE LIFE At least 24 months from the date of manufacture in the original sealed container at ambient temperature. Store away from excessive heat and humidity in tightly closed containers. HANDLING PRECAUTIONS Refer to the Material Safety Data Sheet for 2489 curing agent. TYPICAL PROPERTIES Appearance Clear Liquid Color 1 (Gardner) 1-2 Viscosity 2 @ 77 F (cp) 8 Amine Value 3 (mg KOH/g) 36 Specific Gravity 4 @ 77 F 1.4 Flash Point (closed cup) ( F) 23 Equivalent Wt/{H} 83 Recommended Use Level (phr, EEW=19) 44 TYPICAL HANDLING PROPERTIES A* B* Use Level (phr) 44 41 Mixed Viscosity 2 @ 77 F (cp) 86 8 Gel Time 6 (min) (1 g mix @ 77 F) 32 41 (1 g mix @ F) 16 136 Thin Film Set Time 7 @ 77 F (hr) 3. 4. @ F 8. 13. @ 4 F 1 16 Peak Exotherm 8 (1 g mix @ 77 F) ( F) 2 TYPICAL PERFORMANCE (7 day cure @ 77 F) A* B* Glass Transition Temp 9 ( F) 118 111 Compressive Strength @ yield 1 (psi) 11,7 1,1 Compressive Modulus 1 (thousand psi) 33 28 Tensile Strength 11 (psi) 1, 9,4 Tensile Modulus 11 (thousand psi) 62 Tensile Elongation 11 @ break (%) 2.3.6 Flexural Strength 12 (psi) 19,6 17,9 Flexural Modulus 12 (thousand psi) 787 82 Hardness 13 (Shore D) 8 84 6 Specular Gloss @ 77 F 14 126 123 6 Specular Gloss @ 4 F 14 92 88 A* 2489 formulated with standard bisphenol-a (DGEBA, EEW=19) resin B* 2489 with 9% bis-a resin (EEW=19) and 1% Epodil 748 diluent (C 12 C 14 alkyl glycidyl ether) TYPICAL CURE SCHEDULE 2 7 days at ambient temperature. Note: Please see last page for footnotes. Air Products and Chemicals, Inc., 721 Hamilton Boulevard, Allentown, PA 1819-11 Tel: (8) 34-3148, (61) 481-6799, Fax: (61) 481-4381, http://www.airproducts.com/epoxyadditives The information contained herein is offered without charge for use by technically qualified personnel at their discretion and risk. All statements, technical information and recommendations contained herein are based on tests and data which we believe to be reliable, but the accuracy or completeness thereof is not guaranteed and no warranty of any kind is made with respect thereto. Pub. No. 12-9834

SUPPLEMENTARY INFORMATION Low Mixed Viscosity 2489 curing agent has a viscosity of 8 cp, which is lower than typical modified cycloaliphatic curing agents. Because of its low viscosity and excellent compatibility with epoxy resins, 2489 curing agent gives a mixed viscosity of 86 cp with standard bis-a resin. Low mixed viscosity is a benefit in many applications, such as flooring and mortars, because it promotes easier handling of the final product. The mixed viscosity provided by 2489 is the lowest for the modified cycloaliphatic curing agents Air Products now offers. As shown in Table 1, the mixed viscosity of 2489 curing agent with straight resin is lower than that of many other modified cycloaliphatics, such as 1618 or 2423 curing agents, with 1% diluted resin. Table 1 Mixed Viscosity of Selected Cycloaliphatic Curing Agents 1618 2423 2489 With 9% Bis-A With 1% Bis- Resin/1% Epodil A Resin 748 Diluent Blend 2,4 cp 1,37 cp 4,28 cp 2,2 cp 86 cp 8 cp 2489 curing agent can provide cost effectiveness in epoxy formulations compared with standard modified cycloaliphatic curing agents. The low mixed viscosity of 2489 can give a lower cost in use because it allows higher filler loading and/or reduced use of reactive diluents in the formulated system. Using less diluent in the formulation also results in less of an impact on some performance properties, such as cure speed and chemical resistance, that can be affected by reactive diluent addition. Fast Cure Speed 2489 curing agent provides fast cure and property development at ambient and low temperatures without accelerators, allowing application under a range of temperatures, with a quick return to service. The thin film set time of 2489 curing agent with bis-a based liquid resin in a 3-mil film is 3. hours at 77 F, and 8. hours at F. Cure speed is faster than with most cycloaliphatic curing agents. Figure 1 shows the thin film set time of 2489 versus cycloaliphatic curing agents, 1618 and 2286, with bis-a based liquid resin at 77 F and 4 F. Thin Film Set Time (hr.) 2 1 1 Figure 1 - Thin Film Set Time Comparison 77 F 4 F Cure Temperature 1618 2286 2489 2489 curing agent provides a fast cure with longer working life than other fast curing agents. Figure 2 compares the gel time and thin film set time (TFST) of 2489 with 2368 and 2423 cycloaliphatic curing agents when formulated with standard bisphenol-a resin. TFST at 77 F (hr.) 6 4 3 2 1 Figure 2 - Set Time / Pot Life Balance 2368 TFST 2423 2489 Gel Time 3 3 2 2 1 1 Gel Time (min.) Thin film set time, which is an indicator of the time for an applied coating to set, is 2 hours faster with 2489 than with 2368 curing agent, while gel time, which is an indicator of pot life in a mixing container, is the same at 32 minutes. Compared with 2423 curing agent, 2489 gives almost twice the working time--32 minutes vs. 17 minutes--with the same 3-hour set time. This allows a fast return to service while giving the applicator more time to apply the formulated product after mixing.

Rapid Hardness Development Gel time and thin film set time define the development of cure well, but often do not accurately predict development of hardness. Shore D hardness development was measured as a function of 77 F and 4 F cure for a 1/4-inch thick casting. The results are presented in Table 2. Table 2 2489 Hardness Development Number of Days Cure 1 3 7 77 F Cure Shore D Hardness 13 83 NT 8 4 F Cure Shore D Hardness 13 7 8 Note: 2489 formulated with bis-a (EEW=19) resin. The fast cure and rapid hardness development of formulations cured with 2489 curing agent make it ideal for flooring, coatings and mortars applied at ambient or low temperatures. Even at a temperature as low as 4 F, 2489 curing agent gives a Shore D hardness of within 24 hours. This indicates that it is possible to formulate a system with this product that gives an overnight walk-on at normal temperatures and a oneday walk-on time at low temperatures. Waterspot Resistance Waterspotting can be caused by water drops contacting a coating before it is cured. 2489 curing agent was tested for waterspot resistance in formulations with both undiluted bis-a based resin and 9% bis-a based resin/1% Epodil 748 diluent blend. 1-mil films of each formulation were cured for eight hours at 77 F and % relative humidity. After eight hours, a cotton ball saturated with water was placed on the films. The films were then placed in the incubator for another 24 hours at 77 F and % relative humidity. After this period, the films were examined for white spots. The 2489 formulations showed an absence of spots, indicating very good waterspot resistance at ambient cure conditions. 2489 curing agent was also tested for waterspot resistance at low cure temperatures. A 1-mil film of 2489 with bis-a based resin was cured for 24 hours at 4 F and 9% relative humidity. After 24 hours, a cotton ball saturated with water was placed on the film. The film was then placed in the incubator for 24 hours at 4 F and 9% relative humidity. The film showed minimal waterspotting. Most amine-based curing agents waterspot severely under these aggressive conditions, but 2489 curing agent gives good waterspot resistance. If even faster thin film set and hardness development are needed, 2489 curing agent can be accelerated with fast modified aliphatic amine curing agents such as 289M, 2432, 22 or 186 curing agents. Blush Resistance 2489 curing agent gives high-gloss films with very low or no amine blush when cured at ambient and low temperatures. When combined with standard bis-a resin, the product gives a very high 6 gloss of 126 when cured at 77 F. High gloss at ambient cure is typical of most modified cycloaliphatic curing agents, but 2489 curing agent maintains its high gloss and good film appearance characteristics even under low temperature conditions. When formulated with bis-a resin and cured at 4 F, the film is smooth and clear with a 6 gloss of 92. Most other fast curing hardeners show amine blush and film haziness under low temperature cure conditions.

Chemical Resistance Chemical immersion studies following ASTM D43 were performed on coupons using standard bis-a (DGEBA, EEW=19) liquid resin cured with 2489 curing agent for 7 days at 77 F. Three samples were tested for each reagent. Table 3 shows the average percentage weight change after 3 days and 28 days immersion in various chemicals at 77 F. Spillage resistance studies were conducted on 2489 curing agent formulated with a 9% bis-a resin (EEW=19) and 1% Epodil 748 diluent (C12-C14 alkyl glycidyl ether) blend. Samples were cured for 7 days at 77 F before testing; three samples were tested for each reagent. The immersion/recovery schedule for the testing is shown in Table 4. Percentage weight change and Shore D hardness were measured after each of the immersion periods. The samples were then allowed to recover before reimmersion for the next time period. Hardness retention is relevant in flooring applications where it indicates the ability of the floor to support traffic after exposure to chemical spills. The results of this study are presented in Table. These studies show that 2489 curing agent imparts good resistance to a variety of chemicals. The chemical resistance of 2489-cured formulations can be optimized for specific chemicals using different resin blends, such as bisphenol-f and multifunctional novolac resins. For information on the chemical resistance of many other Air Products curing agents, please refer to our brochure, Chemical Resistance for Ambient Cure Epoxy Formulations. Table 3 Chemical Resistance for 2489 Formulation % Weight Change as a Function of Time (Continuous Immersion) Reagent 2489 / Bis-A Resin After 3 days After 28 days % wt. Change % wt. change Deionized Water.42 1.43 Methanol 1.6 Destroyed Ethanol 3.47 1.2 Toluene 3.1 1.4 Xylene.12.6 Butyl Cellosolve 2.91 7.1 Methyl Ethyl Ketone 11.6 Destroyed 1% Lactic Acid 2.1.82 1% Acetic Acid 3.3 9.2 7% Sulfuric Acid.24-2.4 98% Sulfuric Acid Destroyed % Sodium Hydroxide.9.86 Bleach.43 1.42 Trichloroethane.4.23 Note: Samples cured for 7 days at 77 F before testing. They were tested in accordance with ASTM D43-84.

Table 4 Spillage Resistance Test Method Schedule Castings of 1/8" thickness are immersed for a specified time period. Sample is then removed, weighed and hardness is tested immediately. Sample is then allowed to recover for specified time before re-immersion. 3 hr immersion test 24 hr recovery 24 hr immersion test 24 hr recovery 3 day immersion test 3 day recovery 7 day immersion test 7 day recovery 28 day immersion test 7 day recovery 9 day immersion test Table Spillage Resistance for 2489 with 9% Bis-A Resin / 1% Epodil 748 % Weight Change and Shore D Hardness as a Function of Time REAGENT Initial Test After 3 hr. Test After 24 hr. Test After 3 days Test After 7 days Test After 28 days Test After 9 days 1% Acetic Acid 1% Lactic Acid Toluene Xylene Trichloroethane Methanol Ethanol Butyl Cellosolve Methyl Ethyl Ketone Skydrol 7% Sulfuric Acid Hard. % wt. Hard. % wt. Hard. % wt. Hard. % wt. Hard. % wt. Hard. % wt. Hard. 84.33 81 1.1 7 2.3 74 3. 73.4 69 7.1 6 84.14 83.7 81 1.3 81 2.9 79 3.1 74 3.98 7 84. 8.76 74 3.77 69 8.7 64 1.4 6 19. 48 84. 8.1 77.3 7 1.28 71 4.2 67 6.89 62 84.27 78.6 76 2. 73 6.2 68 12.2 64 18.6 61 84 3.16 67 8. 4 6.9 29 Destroyed 84 1.4 76 2.61 73 4.96 7 8. 62 7.4 7.96 4 84.24 79 1. 7 3. 68.4 63 6.78 6 1. 84 6.46 61 Destroyed 84.4 78.9 78.28 77.71 77.94 7 1.2 7 84.8 82. 81. 82.6 8.11 8.12 79 98% Sulfuric Acid 84-14.18 76 Destroyed Deionized Water % Sodium Hydroxide Bleach 84.1 84.23 84.49 83.81 83 1.13 83 1.2 82 84.7 82 -.4 82 -.7 81 -.1 8 -.9 78 -.12 7 84.24 81. 82.8 81.11 82.24 8.38 78 Note: Samples were cured for 7 days at 77 F before testing. Footnotes 1 ASTM D 144-8 2 ASTM D-44-83, Brookfield, RVTD, Spindle 4 3 Perchloric Acid Titration 4 ASTM D 147-8 Seta Flash Closed Cup 6 Techne GT-4 Gelation Timer 7 BK Drying Recorder 8 ASTM D 2471-71 9 ASTM D 3418-82 1 ASTM D 69-8 11 ASTM D 638-86 12 ASTM D 79-86 13 ASTM D 224-86 14 ASTM D 23-8